Photon Conversion and Interaction in a Quasi-Phase-Matched Microresonator

The conversion and interaction between quantum signals at the single-photon level are essential for scalable quantum photonic information technology. Using a fully optimized periodically poled lithium niobate microring, we demonstrate ultraefficient sum-frequency generation on a chip. The external quantum efficiency reaches (65 +/- 3)% with only (104 +/- 4)-mu W pump power. At peak conversion, 3 x 10(-5)-noise photon is created during the cavity lifetime, which meets the requirement of quantum applications using single-photon pulses. Using a pump and signal in single-photon coherent states, we directly measure the conversion probability produced by a single pump photon to be 10(-5), which is a significant improvement from the state of the art, and the photon-photon coupling strength to be 9.1 MHz. Our results mark steady progress toward quantum nonlinear optics at the ultimate single-photon limit, with potential applications in highly integrated photonics and quantum optical computing.