Attoclock reveals natural coordinates of the laser-induced tunnelling current flow in atoms

被引:362
作者
Pfeiffer, Adrian N. [1 ]
Cirelli, Claudio [1 ]
Smolarski, Mathias [1 ]
Dimitrovski, Darko [2 ]
Abu-samha, Mahmoud [2 ]
Madsen, Lars Bojer [2 ]
Keller, Ursula [1 ]
机构
[1] ETH, Dept Phys, CH-8093 Zurich, Switzerland
[2] Aarhus Univ, Dept Phys & Astron, Lundbeck Fdn Theoret Ctr Quantum Syst Res, DK-8000 Aarhus C, Denmark
基金
瑞士国家科学基金会;
关键词
ATTOSECOND ANGULAR STREAKING; ORDER HARMONIC-GENERATION; RARE-GASES; IONIZATION; FIELD; INTENSE; PULSES; DELAY;
D O I
10.1038/nphys2125
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
In the research area of strong-laser-field interactions and attosecond science(1), tunnelling of an electron through the barrier formed by the electric field of the laser and the atomic potential is typically assumed to be the initial key process that triggers subsequent dynamics(1-3). Here we use the attoclock technique(4) to obtain experimental information about the electron tunnelling geometry (the natural coordinates of the tunnelling current flow) and exit point. We confirm vanishing tunnelling delay time, show the importance of the inclusion of Stark shifts(5,6) and report on multi-electron effects clearly identified by comparing results in argon and helium atoms. Our combined theory and experiment allows us to single out the geometry of the inherently one-dimensional tunnelling problem, through an asymptotic separation of the full three-dimensional problem. Our findings have implications for laser tunnel ionization in all atoms and in particular in larger molecular systems with correspondingly larger dipoles and polarizabilities.
引用
收藏
页码:76 / 80
页数:5
相关论文
共 30 条
[1]   Polarization Effects in Attosecond Photoelectron Spectroscopy [J].
Baggesen, Jan Conrad ;
Madsen, Lars Bojer .
PHYSICAL REVIEW LETTERS, 2010, 104 (04)
[2]   Internal laser-induced dipole force at work in C60 molecule -: art. no. 203004 [J].
Bhardwaj, VR ;
Corkum, PB ;
Rayner, DM .
PHYSICAL REVIEW LETTERS, 2003, 91 (20)
[3]   Intense few-cycle laser fields: Frontiers of nonlinear optics [J].
Brabec, T ;
Krausz, F .
REVIEWS OF MODERN PHYSICS, 2000, 72 (02) :545-591
[4]   Attosecond photon sources: the first decade and beyond [J].
Chang, Zenghu ;
Corkum, P. .
JOURNAL OF THE OPTICAL SOCIETY OF AMERICA B-OPTICAL PHYSICS, 2010, 27 (11) :B9-B17
[5]   PLASMA PERSPECTIVE ON STRONG-FIELD MULTIPHOTON IONIZATION [J].
CORKUM, PB .
PHYSICAL REVIEW LETTERS, 1993, 71 (13) :1994-1997
[6]   Strong-field ionization of polar molecules: Stark-shift-corrected strong-field approximation [J].
Dimitrovski, D. ;
Martiny, C. P. J. ;
Madsen, L. B. .
PHYSICAL REVIEW A, 2010, 82 (05)
[7]   Cold Target Recoil Ion Momentum Spectroscopy:: a 'momentum microscope' to view atomic collision dynamics [J].
Dörner, R ;
Mergel, V ;
Jagutzki, O ;
Spielberger, L ;
Ullrich, J ;
Moshammer, R ;
Schmidt-Böcking, H .
PHYSICS REPORTS-REVIEW SECTION OF PHYSICS LETTERS, 2000, 330 (2-3) :95-192
[8]   Attosecond Ionization and Tunneling Delay Time Measurements in Helium [J].
Eckle, P. ;
Pfeiffer, A. N. ;
Cirelli, C. ;
Staudte, A. ;
Doerner, R. ;
Muller, H. G. ;
Buettiker, M. ;
Keller, U. .
SCIENCE, 2008, 322 (5907) :1525-1529
[9]   Attosecond angular streaking [J].
Eckle, Petrissa ;
Smolarski, Mathias ;
Schlup, Philip ;
Biegert, Jens ;
Staudte, Andre ;
Schoeffler, Markus ;
Muller, Harm G. ;
Doerner, Reinhard ;
Keller, Ursula .
NATURE PHYSICS, 2008, 4 (07) :565-570
[10]   Generation of intense, carrier-envelope phase-locked few-cycle laser pulses through filamentation [J].
Hauri, CP ;
Kornelis, W ;
Helbing, FW ;
Heinrich, A ;
Couairon, A ;
Mysyrowicz, A ;
Biegert, J ;
Keller, U .
APPLIED PHYSICS B-LASERS AND OPTICS, 2004, 79 (06) :673-677