Universal scaling relations for the thermoelectric power factor of semiconducting nanostructures

被引:23
作者
Cornett, Jane E. [1 ]
Rabin, Oded [1 ,2 ]
机构
[1] Univ Maryland, Dept Mat Sci & Engn, College Pk, MD 20742 USA
[2] Univ Maryland, Inst Res Elect & Appl Phys, College Pk, MD 20742 USA
来源
PHYSICAL REVIEW B | 2011年 / 84卷 / 20期
关键词
BISMUTH-ANTIMONY TELLURIDE; THIN METALLIC-FILMS; FIGURE-OF-MERIT; ELECTRON-MOBILITY; QUANTUM-WELL; SILICON NANOWIRES; INVERSION-LAYERS; BULK ALLOYS; SUPERLATTICES; PERFORMANCE;
D O I
10.1103/PhysRevB.84.205410
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
We present a parametric analysis of the thermoelectric power factor of single-carrier semiconductors for nanowires, thin films, and bulk. We consistently find a reduction in the peak power factor in many-subband nanostructures compared to bulk, independent of the specific materials parameters, system geometry, or dimensionality. A universal relation between the optimal power factor and the system size, common to all single-carrier materials, is developed for nanowires and thin films. The common nonmonotonic trend highlights the competing effects of quantization and degeneracy on the transport properties of semiconductor nanostructures. The model predicts decreases of up to 28% and 22% in the peak power factor in nanowires and thin films, respectively, relative to the bulk value. This study provides insights to successful figure-of-merit enhancement strategies.
引用
收藏
页数:10
相关论文
共 42 条
[1]  
Ashcroft N., 2011, Solid State Physics
[2]   Silicon nanowires as efficient thermoelectric materials [J].
Boukai, Akram I. ;
Bunimovich, Yuri ;
Tahir-Kheli, Jamil ;
Yu, Jen-Kan ;
Goddard, William A., III ;
Heath, James R. .
NATURE, 2008, 451 (7175) :168-171
[3]   Thermoelectric transport in quantum well superlattices [J].
Broido, DA ;
Reinecke, TL .
APPLIED PHYSICS LETTERS, 1997, 70 (21) :2834-2836
[4]   Thermoelectric power factor in superlattice systems [J].
Broido, DA ;
Reinecke, TL .
APPLIED PHYSICS LETTERS, 2000, 77 (05) :705-707
[5]  
Broido DA, 2001, SEMICONDUCT SEMIMET, V71, P123
[6]   Theory of thermoelectric power factor in quantum well and quantum wire superlattices [J].
Broido, DA ;
Reinecke, TL .
PHYSICAL REVIEW B, 2001, 64 (04)
[7]   Nanostructured Bulk Silicon as an Effective Thermoelectric Material [J].
Bux, Sabah K. ;
Blair, Richard G. ;
Gogna, Pawan K. ;
Lee, Hohyun ;
Chen, Gang ;
Dresselhaus, Mildred S. ;
Kaner, Richard B. ;
Fleurial, Jean-Pierre .
ADVANCED FUNCTIONAL MATERIALS, 2009, 19 (15) :2445-2452
[8]   Thermoelectric figure of merit calculations for semiconducting nanowires [J].
Cornett, Jane E. ;
Rabin, Oded .
APPLIED PHYSICS LETTERS, 2011, 98 (18)
[9]   High performance silicon nanowire field effect transistors [J].
Cui, Y ;
Zhong, ZH ;
Wang, DL ;
Wang, WU ;
Lieber, CM .
NANO LETTERS, 2003, 3 (02) :149-152
[10]   Influence of acoustic phonon confinement on electron mobility in ultrathin silicon on insulator layers [J].
Donetti, L ;
Gámiz, F ;
Rodriguez, N ;
Jimenez, F ;
Sampedro, C .
APPLIED PHYSICS LETTERS, 2006, 88 (12)