Quantitative Analysis of Ozone and Nitrogen Oxides Produced by a Low Power Miniaturized Surface Dielectric Barrier Discharge: Effect of Oxygen Content and Humidity Level

被引:64
作者
Abdelaziz, Ayman A. [1 ]
Ishijima, Tatsuo [2 ]
Osawa, Naoki [3 ]
Seto, Takafumi [4 ]
机构
[1] Assiut Univ, Phys Dept, Fac Sci, Assiut, Egypt
[2] Kanazawa Univ, Res Ctr Sustainable Energy & Technol, Kakuma Machi, Kanazawa, Ishikawa, Japan
[3] Kanazawa Inst Technol, Dept Elect & Elect Engn, Ctr Elect Opt & Energy Applicat, Nonoichi, Ishikawa, Japan
[4] Kanazawa Univ, Sch Nat Syst, Kakuma Machi, Kanazawa, Ishikawa, Japan
关键词
Surface dielectric barrier discharge; Ozone production; Nitrogen oxides production; Effect of oxygen content; Effect of humidity; Role of excited species; CORONA DISCHARGE; PLASMA; AIR; REMOVAL; GAS; DECOMPOSITION; CONVERSION; REDUCTION; NOX; ACTUATOR;
D O I
10.1007/s11090-018-9942-y
中图分类号
TQ [化学工业];
学科分类号
0817 ;
摘要
This study presented a quantitative evaluation of the performance of a low power miniaturized SDBD source for the production of ozone and nitrogen oxides as benchmarks of long-lived RONS. The effects of varying oxygen and humidity on the trend of the production efficiency are investigated. The oxygen content and the humidity had no noticeable effect on the total power consumed, but their level in the feeding gas has a strong impact on the production of NxOy. It is found also that there is an optimum level of the oxygen content and the humidity for the production of NO2 and N2O. The analysis of the results indicated that the nitrogen excited species, especially N2)" open="and N(D-2) play vital roles in the production of the nitrogen oxides, particularly the NO, which considered as the main source for the other NxOy in the present system. Interestingly, it is found that the humidity has a positive effect on the NO2 production, while it has a negative effect on the N2O and O-3, which implied that the present SDBD is a strong oxidizer for the formed NO. The rise in the gas temperature in the present SDBD was negligible and has no effect on the production of nitrogen oxides, while the temperature of the plasma channel might affect the RONS production efficiency. Investigating the production mechanisms and the energy efficiency, of the formed nitrogen oxides, unravels for the first time the performance of the SDBD for nitrogen fixation.
引用
收藏
页码:165 / 185
页数:21
相关论文
共 79 条
[1]   Humidity effects on surface dielectric barrier discharge for gaseous naphthalene decomposition [J].
Abdelaziz, Ayman A. ;
Ishijima, Tatsuo ;
Seto, Takafumi .
PHYSICS OF PLASMAS, 2018, 25 (04)
[2]   Characterization of surface dielectric barrier discharge influenced by intermediate frequency for ozone production [J].
Abdelaziz, Ayman A. ;
Ishijima, Tatsuo ;
Seto, Takafumi ;
Osawa, Naoki ;
Wedaa, Hassan ;
Otani, Yoshio .
PLASMA SOURCES SCIENCE & TECHNOLOGY, 2016, 25 (03)
[3]   Influence of N2/O2 Mixtures on Decomposition of Naphthalene in Surface Dielectric Barrier Discharge Based Reactor [J].
Abdelaziz, Ayman A. ;
Seto, Takafumi ;
Abdel-Salam, M. ;
Otani, Yoshio .
PLASMA CHEMISTRY AND PLASMA PROCESSING, 2014, 34 (06) :1371-1385
[4]   Performance of a surface dielectric barrier discharge based reactor for destruction of naphthalene in an air stream [J].
Abdelaziz, Ayman A. ;
Seto, Takafumi ;
Abdel-Salam, M. ;
Otani, Yoshio .
JOURNAL OF PHYSICS D-APPLIED PHYSICS, 2012, 45 (11)
[5]   Evaluated kinetic and photochemical data for atmospheric chemistry:: Volume I -: gas phase reactions of Ox, HOx, NOx and SOx species [J].
Atkinson, R ;
Baulch, DL ;
Cox, RA ;
Crowley, JN ;
Hampson, RF ;
Hynes, RG ;
Jenkin, ME ;
Rossi, MJ ;
Troe, J .
ATMOSPHERIC CHEMISTRY AND PHYSICS, 2004, 4 :1461-1738
[6]   Electrical and mechanical characteristics of surface AC dielectric barrier discharge plasma actuators applied to airflow control [J].
Benard, Nicolas ;
Moreau, Eric .
EXPERIMENTS IN FLUIDS, 2014, 55 (11)
[7]   Dielectric barrier discharges: progress on plasma sources and on the understanding of regimes and single filaments [J].
Brandenburg, Ronny .
PLASMA SOURCES SCIENCE & TECHNOLOGY, 2017, 26 (05)
[8]   Inactivation of aquatic microorganisms by low-frequency AC discharges [J].
Chen, Chih Wei ;
Lee, How-Ming ;
Chang, Moo Been .
IEEE TRANSACTIONS ON PLASMA SCIENCE, 2008, 36 (01) :215-219
[9]   Effect of relative humidity on electron distribution and ozone production by DC coronas in air [J].
Chen, JH ;
Wang, PX .
IEEE TRANSACTIONS ON PLASMA SCIENCE, 2005, 33 (02) :808-812
[10]  
Chiper AS, 2006, J OPTOELECTRON ADV M, V8, P208