Low-temperature properties of Ca-doped YbMnO3 multiferroic single crystals

被引:12
作者
Abramov, N. [1 ]
Chichkov, V. [1 ]
Lofland, S. E. [2 ]
Mukovskii, Y. M. [1 ]
机构
[1] Natl Univ Sci & Technol MISiS, Moscow 119049, Russia
[2] Rowan Univ, Glassboro, NJ 08028 USA
基金
美国国家科学基金会;
关键词
MAGNETIC PHASE-DIAGRAMS; YMNO3; HEAT;
D O I
10.1063/1.3556961
中图分类号
O59 [应用物理学];
学科分类号
摘要
The specific heat c(p) and magnetization of single crystal hexagonal manganites of the type Yb1-xCaxMnO3 (x = 0, 0.05, and 0.10) were measured in a wide temperature range as a function of magnetic field. Antiferromagnetic ordering of the Mn sublattice occurs at T-N = 83 K. Ca doping has surprisingly minimal effect on the magnetic properties. At low temperature (similar to 3.5 K), all compounds show ferromagnetic (FM) ordering in the basal plane attributed to Yb in site 2a. For low fields applied along the c direction, Yb spin reorientation occurs and FM ordering disappears. cp shows a broad maximum centered at the temperature similar to 6 K that is consistent with a Schottky anomaly related to the Zeeman splitting of the Yb moments due to Mn molecular field. In the field of 30 kOe, the re-entrant FM transition takes place with Yb ions in sites 2a and 4b. (C) 2011 American Institute of Physics. [doi:10.1063/1.3556961]
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页数:3
相关论文
共 14 条
[1]   Ferroelectricity and structure in the YMnO3 family [J].
Abrahams, SC .
ACTA CRYSTALLOGRAPHICA SECTION B-STRUCTURAL SCIENCE, 2001, 57 (04) :485-490
[2]   Magnetic order in YbMnO3 studied by neutron diffraction and Mossbauer spectroscopy [J].
Fabreges, X. ;
Mirebeau, I. ;
Bonville, P. ;
Petit, S. ;
Lebras-Jasmin, G. ;
Forget, A. ;
Andre, G. ;
Pailhes, S. .
PHYSICAL REVIEW B, 2008, 78 (21)
[3]   Determination of the magnetic symmetry of hexagonal manganites by second harmonic generation [J].
Fiebig, M ;
Fröhlich, D ;
Kohn, K ;
Leute, S ;
Lottermoser, T ;
Pavlov, VV ;
Pisarev, RV .
PHYSICAL REVIEW LETTERS, 2000, 84 (24) :5620-5623
[4]   Spin-rotation phenomena and magnetic phase diagrams of hexagonal RMnO3 [J].
Fiebig, M ;
Lottermoser, T ;
Pisarev, RV .
JOURNAL OF APPLIED PHYSICS, 2003, 93 (10) :8194-8196
[5]   Magnetic response of YbMnO3 single crystal [J].
Fontcuberta, Josep ;
Gospodinov, Marin ;
Skumryev, Vassil .
JOURNAL OF APPLIED PHYSICS, 2008, 103 (07)
[6]   Low temperature transport and specific heat studies of Nd1-xPbxMnO3 single crystals [J].
Ghosh, N. ;
Roessler, U. K. ;
Nenkov, K. ;
Hucho, C. ;
Bhat, H. L. ;
Mueller, K-H .
JOURNAL OF PHYSICS-CONDENSED MATTER, 2008, 20 (39)
[7]  
GOPAL ESR, 1966, SPECIFIC HEATS LOW T, P31
[8]   Specific heat of Nd0.67Sr0.33MnO3 [J].
Gordon, JE ;
Fisher, RA ;
Jia, YX ;
Phillips, NE ;
Reklis, SF ;
Wright, DA ;
Zettl, A .
PHYSICAL REVIEW B, 1999, 59 (01) :127-130
[9]   High-temperature structural evolution of hexagonal multiferroic YMnO3 and YbMnO3 [J].
Jeong, Il-Kyoung ;
Hur, N. ;
Proffen, Th. .
JOURNAL OF APPLIED CRYSTALLOGRAPHY, 2007, 40 :730-734
[10]   Dielectric and magnetic anomalies and spin frustration in hexagonal RMnO3 (R = Y, Yb, and Lu) -: art. no. 104419 [J].
Katsufuji, T ;
Mori, S ;
Masaki, M ;
Moritomo, Y ;
Yamamoto, N ;
Takagi, H .
PHYSICAL REVIEW B, 2001, 64 (10)