Greenhouse gas emission estimation from municipal wastewater using a hybrid approach of generative adversarial network and data-driven modelling

Greenhouse gas (GHG) emissions including carbon dioxide (CO2), methane (CH4), and nitrous oxide (N2O) created via wastewater treatment processes are not easily modeled given the non-linearity and complexity of biological processes. These factors are also impacted by limited data availability making the development of artificial data generation algorithms, such as a generative adversarial network (GAN), useful for determination of GHG emission rate estimates (EREs). The main objective of this study was to develop a hybrid approach of using GAN and regression modelling to determine GHG EREs from a cold-region biological nutrient removal (BNR) municipal wastewater treatment plant (MWTP) in which the aerobic reactor has previously been established as the main GHG emission source. To our knowledge, this is the first application of GAN used for MWTP modelling purposes. The EREs were generated from laboratory-scale reactors used in conjunction with facility-monitored operating parameters to develop the GAN and regression models. Results showed that regression models provided reasonable EREs using parameters including hydraulic retention time (HRT), temperature, total organic carbon, and dissolved oxygen (DO) concentrations for CO2 EREs; HRT, temperature, DO and phosphate (PO43-) concentrations for CH4 EREs; and temperature, DO, and nitrogen (nitrite, nitrate, and ammonium) concentrations for N2O EREs. Additionally, the addition of 100 GAN-created virtual data points improved regression model metrics including increased correlation coefficient and index agreement values, and decreased root mean square error values. Clearly, virtual data augmentation using GAN is a valuable resource in supplementation of limited data for improved modelling outcomes. Genetic algorithm optimization was also used to determine operating parameter modifications resulting in potential for minimization (or maximization) of GHG emissions. (C) 2021 Elsevier B.V. All rights reserved.