Wildfire Impact on Indoor and Outdoor PAH Air Quality

被引:35
作者
Ghetu, Christine C. [1 ]
Rohlman, Diana [2 ]
Smith, Brian W. [1 ]
Scott, Richard P. [1 ]
Adams, Kaley A. [1 ]
Hoffman, Peter D. [1 ]
Anderson, Kim A. [1 ]
机构
[1] Oregon State Univ, Dept Environm & Mol Toxicol, Corvallis, OR 97331 USA
[2] Oregon State Univ, Coll Publ Hlth & Human Sci, Corvallis, OR 97331 USA
关键词
passive sampling; vapor-phase PAHs; public health; community-engaged research; wildfire PAH exposure mixture; POLYCYCLIC AROMATIC-HYDROCARBONS; EXPOSURE; GAS; EMISSIONS; POLLUTION; POLLUTANTS; PHASES; MATTER; CITIES; URBAN;
D O I
10.1021/acs.est.2c00619
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
ABSTRACT: Air quality impacts from wildfires are poorly understood, particularly indoors. As frequencies increase, it is important to optimize methodologies to understand and reduce chemical exposures from wildfires. Public health recommendations use air quality estimates from outdoor stationary air monitors, discounting indoor air conditions, and do not consider chemicals in the vapor phase, known to elicit adverse effects. We investigated vapor-phase polycyclic aromatic hydrocarbons (PAHs) in indoor and outdoor air before, during, and after wildfires using a community-engaged research approach. Paired passive air samplers were deployed at 15 locations across four states. Twelve unique PAHs were detected only in outdoor air during wildfires, highlighting a PAH exposure mixture for future study. Heavy-molecular-weight (HMW) outdoor PAH concentrations and average Air Quality Index (AQI) values were positively correlated (p < 0.001). Indoor PAH concentrations were higher in 77% of samples across all sampling events. Even during wildfires, 58% of sampled locations still had higher indoor PAH air concentrations. When AQI values exceeded 140 (unhealthy for sensitive groups), outdoor PAH concentrations became similar to or higher than indoors. Cancer and noncancer inhalation risk estimates from vapor-phase PAHs were higher indoors than outdoors, regardless of the wildfire impact. Consideration of indoor air quality and vapor-phase PAHs could inform public health recommendations regarding wildfires.
引用
收藏
页码:10042 / 10052
页数:11
相关论文
共 76 条
[1]  
Abdel-Shafy Hussein I., 2016, Egyptian Journal of Petroleum, V25, P107, DOI [10.1016/j.ejpe.2015.03.011, 10.1016/j.ejpe.2015.03.011]
[2]   Fine Particles in Wildfire Smoke and Pediatric Respiratory Health in California [J].
Aguilera, Rosana ;
Corringham, Thomas ;
Gershunov, Alexander ;
Leibel, Sydney ;
Benmarhnia, Tarik .
PEDIATRICS, 2021, 147 (04)
[3]  
airnow, AIRNOW AIR QUALITY I
[4]   Impact of the Deepwater Horizon Oil Spill on Bioavailable Polycyclic Aromatic Hydrocarbons in Gulf of Mexico Coastal Waters [J].
Allan, Sarah E. ;
Smith, Brian W. ;
Anderson, Kim A. .
ENVIRONMENTAL SCIENCE & TECHNOLOGY, 2012, 46 (04) :2033-2039
[5]   Field trial and modeling of uptake rates of in situ lipid-free polyethylene membrane passive sampler [J].
Anderson, K. A. ;
Sethajintanin, D. ;
Sower, G. ;
Quarles, L. .
ENVIRONMENTAL SCIENCE & TECHNOLOGY, 2008, 42 (12) :4486-4493
[6]   Modified ion source triple quadrupole mass spectrometer gas chromatograph for polycyclic aromatic hydrocarbon analyses [J].
Anderson, Kim A. ;
Szelewski, Michael J. ;
Wilson, Glenn ;
Quimby, Bruce D. ;
Hoffman, Peter D. .
JOURNAL OF CHROMATOGRAPHY A, 2015, 1419 :89-98
[7]   Time to Say Goodbye to the 16 EPA PAHs? Toward an Up-to-Date Use of PACs for Environmental Purposes [J].
Andersson, Jan T. ;
Achten, Christine .
POLYCYCLIC AROMATIC COMPOUNDS, 2015, 35 (2-4) :330-354
[8]  
[Anonymous], US Environmental Protection Agency
[9]  
[Anonymous], 2009, Risk Assessment Guidance for Superfund
[10]   Oxidative stress and respiratory symptoms due to human exposure to polycyclic aromatic hydrocarbons (PAHs) in Kumasi, Ghana [J].
Bortey-Sam, Nesta ;
Ikenaka, Yoshinori ;
Akoto, Osei ;
Nakayama, Shouta M. M. ;
Asante, Kwadwo A. ;
Baidoo, Elvis ;
Obirikorang, Christian ;
Saengtienchai, Aksorn ;
Isoda, Norikazu ;
Nimako, Collins ;
Mizukawa, Hazuki ;
Ishizuka, Mayumi .
ENVIRONMENTAL POLLUTION, 2017, 228 :311-320