Multi-residues of organic pollutants in surface sediments from littoral areas of the Yellow Sea, China

被引:24
作者
Liu, WenXin [1 ]
Chen, JiangLin [2 ]
Hu, Jing [1 ]
Ling, Xi [1 ]
Tao, Shu [1 ]
机构
[1] Peking Univ, Coll Urban & Environm Sci, Lab Earth Surface Proc, Beijing 100871, Peoples R China
[2] SOA, N China Sea Branch, Qingdao 266033, Peoples R China
基金
中国国家自然科学基金;
关键词
organic pollutants; surface sediments; distribution; property; Yellow Sea;
D O I
10.1016/j.marpolbul.2008.03.021
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Concentrations of all studied organic pollutants, except for DDTs, were greatest at sites in Dalian Bay, where surface sediment concentrations of PHCs, PAHs, PCBs and DDTs exceeded the corresponding ERL values. The sum concentration of DDTs was greatest in Haizhou Bay exceeding the related ERM value. In terms of compositions of PAHs and PAEs, the predominant components were the MMW and HMW compounds, DBP and DEHP, respectively. The main degradation product of p,p'-DDT was p,p'-DDD at most sampling sites. The principal sources of PAHs and DDTs involved various pyrolytic processes (i.e., combustion of biomass and vehicle exhaust), and application of technical DDT (in the form of impurity or raw material), and a mixture of technical DDT and technical dicofol. Moreover, the coastal site with greatest potential ecological risk from total PAHs was located in Dalian Bay, while the littoral areas of Dalian Bay, two harbor cities (Yantai-Weihai), Jiaozhou Bay, and Haizhou Bay, had relatively high potential risk from DDTs, especially in Haizhou Bay. (C) 2008 Elsevier Ltd. All rights reserved.
引用
收藏
页码:1091 / 1103
页数:13
相关论文
共 44 条
[21]   The sediment quality guideline, ERL, is not a chemical concentration at the threshold of sediment toxicity [J].
O'Connor, TP .
MARINE POLLUTION BULLETIN, 2004, 49 (5-6) :383-385
[22]   A preliminary report of persistent orgranochlorine pollutants in the Yellow Sea [J].
Oh, JR ;
Choi, HK ;
Hong, SH ;
Yim, UH ;
Shim, WJ ;
Kannan, N .
MARINE POLLUTION BULLETIN, 2005, 50 (02) :217-222
[23]   PCBs, PCNs and PBDEs in sediments and mussels from Qingdao coastal sea in the frame of current circulations and influence of sewage sludge [J].
Pan, Jing ;
Yang, Yong-Liang ;
Xu, Qing ;
Chen, Da-Zhou ;
Xi, Dan-Li .
CHEMOSPHERE, 2007, 66 (10) :1971-1982
[24]   Contribution of dicofol to the current DDT pollution in China [J].
Qiu, XH ;
Zhu, T ;
Yao, B ;
Hu, JX ;
Hu, SW .
ENVIRONMENTAL SCIENCE & TECHNOLOGY, 2005, 39 (12) :4385-4390
[25]   Organochlorine pesticides in the air around the Taihu Lake, China [J].
Qiu, XH ;
Zhu, T ;
Jing, L ;
Pan, HS ;
Li, QL ;
Miao, GF ;
Gong, JC .
ENVIRONMENTAL SCIENCE & TECHNOLOGY, 2004, 38 (05) :1368-1374
[26]   ALIPHATIC AND AROMATIC-HYDROCARBONS IN DIFFERENT SIZED AEROSOLS OVER THE MEDITERRANEAN-SEA - OCCURRENCE AND ORIGIN [J].
SICRE, MA ;
MARTY, JC ;
SALIOT, A ;
APARICIO, X ;
GRIMALT, J ;
ALBAIGES, J .
ATMOSPHERIC ENVIRONMENT, 1987, 21 (10) :2247-2259
[27]  
SOA CHIN, 1999, Patent No. 173781998
[28]  
SOA CHIN, 2002, Patent No. 186682002
[29]   Environmental assessment of polycyclic aromatic hydrocarbons (PAHs) in surface sediments of the Santander Bay, Northern Spain [J].
Viguri, J ;
Verde, J ;
Irabien, A .
CHEMOSPHERE, 2002, 48 (02) :157-165
[30]   Passive air sampling of DDT, chlordane and HCB in the Pearl River Delta, South China: Implications to regional sources [J].
Wang, Jun ;
Guo, Lingli ;
Li, Jun ;
Zhang, Gan ;
Lee, Celine S. L. ;
Li, Xiangdong ;
Jones, Kevin C. ;
Xiang, Yunrong ;
Zhong, Liuju .
JOURNAL OF ENVIRONMENTAL MONITORING, 2007, 9 (06) :582-588