Energy Decarbonization via Green H2 or NH3?

被引：99

作者：

Wu, Simson ^{[1
,2
]}

Salmon, Nicholas ^{[3
]}

Li, Molly Meng-Jung ^{[4
]}

Banares-Alcantara, Rene ^{[3
]}

Tsang, Shik Chi Edman ^{[1
,2
]}

机构：

[1] Oxford Green Innotech Ltd OXGRIN, Oxford OX4 2HN, England

[2] Univ Oxford, Wolfson Catalysis Ctr, Dept Chem, Oxford OX1 3QR, England

[3] Univ Oxford, Dept Engn Sci, Oxford OX1 3PJ, England

[4] Hong Kong Polytech Univ, Dept Appl Phys, Kowloon, Hong Kong 999077, Peoples R China

来源：

ACS ENERGY LETTERS | 2022年 / 7卷 / 03期

关键词：

LIFE-CYCLE ASSESSMENT; AMMONIA-SYNTHESIS; HYDROGEN; STORAGE; WATER; TECHNOLOGIES; EFFICIENT; N-2;

D O I：

10.1021/acsenergylett.1c02816

中图分类号：

O64 [物理化学（理论化学）、化学物理学];

学科分类号：

070304 ; 081704 ;

摘要：

Due to the global need to decarbonize, it is increasingly clear that we are heading toward a new era of massive renewable energy generation and utilization to substitute fossil fuels. However, pragmatic means for renewable energy storage, transportation, and utilization at a very large scale are not yet fully developed and require careful scrutiny. In this Focus Review, we will consider the thermodynamics, kinetic barriers, material challenges, current science and technology readiness, and geographical locations for green hydrogen versus green ammonia as energy vectors for suitable sustainability of our future economy.

引用

页码：1021 / 1033

页数：13

共 107 条

[1]

ABS, 2020, SUST WHIT AMM MAR FU

[2]

Alfa Laval, 2020, Ammonfuel: An industrial view of ammonia as a marine fuel

[3] A rigorous electrochemical ammonia synthesis protocol with quantitative isotope measurements [J].

Andersen, Suzanne Z. ;

Colic, Viktor ;

Yang, Sungeun ;

Schwalbe, Jay A. ;

Nielander, Adam C. ;

McEnaney, Joshua M. ;

Enemark-Rasmussen, Kasper ;

Baker, Jon G. ;

Singh, Aayush R. ;

Rohr, Brian A. ;

Statt, Michael J. ;

Blair, Sarah J. ;

Mezzavilla, Stefano ;

Kibsgaard, Jakob ;

Vesborg, Peter C. K. ;

Cargnello, Matteo ;

Bent, Stacey F. ;

Jaramillo, Thomas F. ;

Stephens, Ifan E. L. ;

Norskov, Jens K. ;

Chorkendorff, Ib .

NATURE, 2019, 570 (7762) :504-+

[4] A ROLE FOR AMMONIA IN THE HYDROGEN ECONOMY [J].

AVERY, WH .

INTERNATIONAL JOURNAL OF HYDROGEN ENERGY, 1988, 13 (12) :761-773

[5] Ammonia as Effective Hydrogen Storage: A Review on Production, Storage and Utilization [J].

Aziz, Muhammad ;

Wijayanta, Agung Tri ;

Nandiyanto, Asep Bayu Dani .

ENERGIES, 2020, 13 (12)

[6]

BARBIR F, 2005, CHEM IND CHEM ENG Q, V11, P105, DOI DOI 10.2298/CICEQ0503105B

[7] On the climate impacts of blue hydrogen production [J].

Bauer, Christian ;

Treyer, Karin ;

Antonini, Cristina ;

Bergerson, Joule ;

Gazzani, Matteo ;

Gencer, Emre ;

Gibbins, Jon ;

Mazzotti, Marco ;

McCoy, Sean T. ;

McKenna, Russell ;

Pietzcker, Robert ;

Ravikumar, Arvind P. ;

Romano, Matteo C. ;

Ueckerdt, Falko ;

Vente, Jaap ;

van der Spek, Mijndert .

SUSTAINABLE ENERGY & FUELS, 2021, 6 (01) :66-75

[8]

Bird F., 2020, The Royal Society

[9] Facts or Artifacts: Pitfalls in Quantifying Sub-ppm Levels of Ammonia Produced from Electrochemical Nitrogen Reduction [J].

Biswas, Suchi Smita ;

Saha, Arunava ;

Eswaramoorthy, Muthusamy .

ACS OMEGA, 2022, 7 (02) :1874-1882

[10] Environmental Life Cycle Assessment of Ammonia-Based Electricity [J].

Boero, Andrea J. ;

Kardux, Kevin ;

Kovaleva, Marina ;

Salas, Daniel A. ;

Mooijer, Jacco ;

Mashruk, Syed ;

Townsend, Michael ;

Rouwenhorst, Kevin ;

Valera-Medina, Agustin ;

Ramirez, Angel D. .

ENERGIES, 2021, 14 (20)

← 1 2 3 4 5 6 7 8 9 10 →