Reduced graphene oxide as co-catalyst for enhanced visible light photocatalytic activity of BiOBr

被引:32
作者
Jiang, Tingting [1 ]
Li, Jinliang [1 ]
Sun, Zhuo [1 ]
Liu, Xinjuan [2 ]
Lu, Ting [1 ]
Pan, Likun [1 ]
机构
[1] East China Normal Univ, Sch Phys & Mat Sci, Minist Educ, Engn Res Ctr Nanophoton & Adv Instrument, Shanghai 200062, Peoples R China
[2] China Jiliang Univ, Coll Mat Sci & Engn, Inst Coordinat Bond Metrol & Engn, Hangzhou, Zhejiang, Peoples R China
基金
中国国家自然科学基金;
关键词
BiOBr; Reduced graphene oxide; Nitrobenzene; Photocatalysis; MICROWAVE-ASSISTED METHOD; ONE-POT SYNTHESIS; SOLVOTHERMAL SYNTHESIS; HIGH-PERFORMANCE; SHELL STRUCTURE; METHYLENE-BLUE; CARBON-FIBERS; 001; FACETS; DEGRADATION; COMPOSITE;
D O I
10.1016/j.ceramint.2016.06.079
中图分类号
TQ174 [陶瓷工业]; TB3 [工程材料学];
学科分类号
0805 ; 080502 ;
摘要
BiOBr-reduced graphene oxide (RGO) composites were successfully synthesized via a simple hydro thermal method. Their morphology, structure and photocatalytic activity in the degradation of nitrobenzene were characterized by scanning electron microscopy, X-ray diffraction, nitrogen adsorption-desorption, UV-vis absorption spectroscopy, photoluminescence spectra, electrochemical impedance spectra and total organic carbon, respectively. The results showed that the introduction of RGO could enhance the visible light photocatalytic activity of BiOBr. The BiOBr-RGO composite with 0.6 wt% RGO exhibited an optimal photocatalytic activity, and the maximum degradation rate of nitrobenzene was about 2.16 times that of pure BiOBr due to the increased light absorption and the reduced electron-hole pair recombination in BiOBr with the introduction of RGO. (C) 2016 Published by Elsevier Ltd and Techna Group S.r.l.
引用
收藏
页码:16463 / 16468
页数:6
相关论文
共 58 条
  • [1] Morphology-dependent photocatalytic removal of NO by hierarchical BiVO4 microboats and microspheres under visible light
    Ai, Zhihui
    Lee, Shuncheng
    [J]. APPLIED SURFACE SCIENCE, 2013, 280 : 354 - 359
  • [2] Efficient Visible Light Photocatalytic Removal of NO with BiOBr-Graphene Nanocomposites
    Ai, Zhihui
    Ho, Wingkei
    Lee, Shuncheng
    [J]. JOURNAL OF PHYSICAL CHEMISTRY C, 2011, 115 (51) : 25330 - 25337
  • [3] Monoclinic α-Bi2O3 photocatalyst for efficient removal of gaseous NO and HCHO under visible light irradiation
    Ai, Zhihui
    Huang, Yu
    Lee, Shuncheng
    Zhang, Lizhi
    [J]. JOURNAL OF ALLOYS AND COMPOUNDS, 2011, 509 (05) : 2044 - 2049
  • [4] Catalysis for CO2 conversion: a key technology for rapid introduction of renewable energy in the value chain of chemical industries
    Centi, Gabriele
    Quadrelli, Elsje Alessandra
    Perathoner, Siglinda
    [J]. ENERGY & ENVIRONMENTAL SCIENCE, 2013, 6 (06) : 1711 - 1731
  • [5] Enhanced photocatalytic performance over Bi4Ti3O12 nanosheets with controllable size and exposed {001} facets for Rhodamine B degradation
    Chen, Zhiwu
    Jiang, Hong
    Jin, Wuliang
    Shi, Chunkai
    [J]. APPLIED CATALYSIS B-ENVIRONMENTAL, 2016, 180 : 698 - 706
  • [6] Visible-Light-Promoted Stereoselective Alkylation by Combining Heterogeneous Photocatalysis with Organocatalysis
    Cherevatskaya, Maria
    Neumann, Matthias
    Fueldner, Stefan
    Harlander, Christoph
    Kuemmel, Susanne
    Dankesreiter, Stephan
    Pfitzner, Arno
    Zeitler, Kirsten
    Koenig, Burkhard
    [J]. ANGEWANDTE CHEMIE-INTERNATIONAL EDITION, 2012, 51 (17) : 4062 - 4066
  • [7] The effects of Fe, Co and Ni dopants on TiO2 structure of sol-gel nanopowders used as photocatalysts for environmental protection: A comparative study
    Crisan, Maria
    Dragan, Nicolae
    Crisan, Dorel
    Ianculescu, Adelina
    Nitoi, Ines
    Oancea, Petruta
    Todan, Ligia
    Stan, Cristina
    Stanica, Nicolae
    [J]. CERAMICS INTERNATIONAL, 2016, 42 (02) : 3088 - 3095
  • [8] Fabrication of hollow inorganic fullerene-like BiOBr eggshells with highly efficient visible light photocatalytic activity
    Deng, Chonghai
    Guan, Hanmin
    [J]. MATERIALS LETTERS, 2013, 107 : 119 - 122
  • [9] (NH4)2CO3 mediated hydrothermal synthesis of N-doped (BiO)2CO3 hollow nanoplates microspheres as high-performance and durable visible light photocatalyst for air cleaning
    Dong, Fan
    Liu, Haitao
    Ho, Wing-Kei
    Fu, Min
    Wu, Zhongbiao
    [J]. CHEMICAL ENGINEERING JOURNAL, 2013, 214 : 198 - 207
  • [10] Novel carbon dots/BiOBr nanocomposites with enhanced UV and visible light driven photocatalytic activity
    Du, Qingqing
    Wang, Wenpeng
    Wu, Yongzhong
    Zhao, Gang
    Ma, Fukun
    Hao, Xiaopeng
    [J]. RSC ADVANCES, 2015, 5 (39): : 31057 - 31063