Catalytic conversion of methane to methanol over Cu-mordenite

被引:192
作者
Alayon, Evalyn Mae [1 ,2 ]
Nachtegaal, Maarten [1 ]
Ranocchiari, Marco [1 ]
van Bokhoven, Jeroen A. [1 ,2 ]
机构
[1] Paul Scherrer Inst, CH-5232 Villigen, Switzerland
[2] Swiss Fed Inst Technol, CH-8093 Zurich, Switzerland
关键词
NITROUS-OXIDE; ACTIVE-SITE; OXIDATION; ZEOLITES; CU-ZSM-5; OXYGEN; BIS(MU-OXO)DICOPPER; DECOMPOSITION; INTERMEDIATE; CHEMISTRY;
D O I
10.1039/c1cc15840f
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Methane can be converted to methanol over copper-exchanged mordenite at 200 degrees C. Methanol could be recovered at the end of the reactor. This multi-step reaction opens the possibility for methane to methanol conversion in a closed catalytic cyclic reaction system.
引用
收藏
页码:404 / 406
页数:3
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