Two-dimensional/one-dimensional molybdenum sulfide (MoS2) nanoflake/graphitic carbon nitride (g-C3N4) hollow nanotube photocatalyst for enhanced photocatalytic hydrogen production activity

被引：107

作者：

Sun, Jiwei ^{[1
]}

Yang, Shaorui ^{[1
]}

Liang, Zhangqian ^{[1
]}

Liu, Xiang ^{[1
]}

Qiu, Pengyuan ^{[1
]}

Cui, Hongzhi ^{[1
]}

Tian, Jian ^{[1
]}

机构：

[1] Shandong Univ Sci & Technol, Sch Mat Sci & Engn, Qingdao 266590, Peoples R China

来源：

JOURNAL OF COLLOID AND INTERFACE SCIENCE | 2020年 / 567卷

基金：

中国国家自然科学基金;

关键词：

g-C3N4; nanotubes; MoS2; nanoflakes; Photocatalytic hydrogen evolution; 1D hollow structure; EXPOSED; 001; FACETS; HETEROJUNCTION PHOTOCATALYSTS; H-2; EVOLUTION; DOPED G-C3N4; NANOSHEETS; FABRICATION;

D O I：

10.1016/j.jcis.2020.02.029

中图分类号：

O64 [物理化学（理论化学）、化学物理学];

学科分类号：

070304 ; 081704 ;

摘要：

The graphitic carbon nitride (g-C3N4) hollow nanotubes synthesized via a simple freeze-drying method are used for constructing Two-dimensional (2D)-one-dimensional (1D) molybdenum sulfide (MoS2) nanoflake/g-C3N4 hollow nanotube (MoS2/g-C3N4 nanotube) photocatalysts. The MoS2/g-C3N4 nanotube composite with 15 wt% MoS2 shows the highest hydrogen (H-2) production rate (1124 mu mol.h(-1).g(-1)), much higher than bulk g-C3N4 (64 mu mol.h(-1).g(-1)) and g-C3N4 nanotubes (189 mu mol.h(-l).g(-1)). The excellent photocatalytic activity of MoS2/g-C3N4 nanotube composites can be ascribed to more exposed active edges of 2D-1D structure, multiple light reflection/scattering channels of 2D nanoflake/1D hollow nanotube composite structure and better carrier transfer and separation by heterojunction interface. (C) 2020 Elsevier Inc. All rights reserved.

引用

页码：300 / 307

页数：8

共 49 条

[1] Scanning Acoustic Microscopy and Time-Resolved Fluorescence Spectroscopy for Characterization of Atherosclerotic Plaques [J].

Bilen, Bukem ;

Gokbulut, Belkis ;

Kafa, Ulku ;

Heves, Emre ;

Inci, Mehmet Naci ;

Unlu, Mehmet Burcin .

SCIENTIFIC REPORTS, 2018, 8

[2] Three-dimensional porous g-C3N4 for highly efficient photocatalytic overall water splitting [J].

Chen, Xianjie ;

Shi, Run ;

Chen, Qian ;

Zhang, Zijian ;

Jiang, Wenjun ;

Zhu, Yongfa ;

Zhang, Tierui .

NANO ENERGY, 2019, 59 :644-650

[3] An alkali treating strategy for the colloidization of graphitic carbon nitride and its excellent photocatalytic performance [J].

Cheng, Fuxing ;

Yan, Jing ;

Zhou, Chenjuan ;

Chen, Binhe ;

Li, Peiran ;

Chen, Zhi ;

Dong, Xiaoping .

JOURNAL OF COLLOID AND INTERFACE SCIENCE, 2016, 468 :103-109

[4] FREUNDLICH, LANGMUIR, TEMKIN AND HARKINS-JURA ISOTHERMS STUDIES OF H2 ADSORPTION ON POROUS ADSORBENTS [J].

Erdogan, Fatma Oguz .

CHEMISTRY & CHEMICAL TECHNOLOGY, 2019, 13 (02) :129-135

[5] g-C3N4-Based Heterostructured Photocatalysts [J].

Fu, Junwei ;

Yu, Jiaguo ;

Jiang, Chuanjia ;

Cheng, Bei .

ADVANCED ENERGY MATERIALS, 2018, 8 (03)

[6] The selective deposition of MoS2 nanosheets onto (101) facets of TiO2 nanosheets with exposed (001) facets and their enhanced photocatalytic H2 production [J].

Hu, Xiaolin ;

Lu, Shucao ;

Tian, Jian ;

Wei, Na ;

Song, Xiaojie ;

Wang, Xinzhen ;

Cui, Hongzhi .

APPLIED CATALYSIS B-ENVIRONMENTAL, 2019, 241 :329-337

[7] Megamerger in photocatalytic field: 2D g-C3N4 nanosheets serve as support of 0D nanomaterials for improving photocatalytic performance [J].

Huang, Danlian ;

Li, Zhihao ;

Zeng, Guangming ;

Zhou, Chengyun ;

Xue, Wenjing ;

Gong, Xiaomin ;

Yan, Xuelei ;

Chen, Sha ;

Wang, Wenjun ;

Cheng, Min .

APPLIED CATALYSIS B-ENVIRONMENTAL, 2019, 240 :153-173

[8] Metal-free efficient photocatalyst for stable visible-light photocatalytic degradation of refractory pollutant [J].

Jiang, Longbo ;

Yuan, Xingzhong ;

Zeng, Guangming ;

Wu, Zhibin ;

Liang, Jie ;

Chen, Xiaohong ;

Leng, Lijian ;

Wang, Hui ;

Wang, Hou .

APPLIED CATALYSIS B-ENVIRONMENTAL, 2018, 221 :715-725

[9] Enhancement of photocatalytic hydrogen evolution activity of porous oxygen doped g-C3N4 with nitrogen defects induced by changing electron transition [J].

Jiang, Yabin ;

Sun, Zongzhao ;

Tang, Chao ;

Zhou, Yuxia ;

Zeng, Lei ;

Huang, Limin .

APPLIED CATALYSIS B-ENVIRONMENTAL, 2019, 240 :30-38

[10] A Hierarchical Z-Scheme α-Fe2O3/g-C3N4 Hybrid for Enhanced Photocatalytic CO2 Reduction [J].

Jiang, Zhifeng ;

Wan, Weiming ;

Li, Huaming ;

Yuan, Shouqi ;

Zhao, Huijun ;

Wong, Po Keung .

ADVANCED MATERIALS, 2018, 30 (10)

← 1 2 3 4 5 →