Field-Effect Device Using Quasi-Two-Dimensional Electron Gas in Mass-Producible Atomic-Layer-Deposited Al2O3/TiO2 Ultrathin (<10 nm) Film Heterostructures

被引:59
作者
Seok, Tae Jun [1 ]
Liu, Yuhang [1 ]
Jung, Hae Jun [3 ,4 ]
Kim, Soo Bin [3 ,4 ]
Kim, Dae Hyun [2 ]
Kim, Sung Min [3 ,4 ]
Jang, Jae Hyuck [5 ]
Cho, Deok-Yong [6 ,7 ]
Lee, Sang Woon [3 ,4 ]
Park, Tae Joo [1 ,2 ]
机构
[1] Hanyang Univ, Dept Mat Sci & Chem Engn, Ansan 15588, South Korea
[2] Hanyang Univ, Dept Adv Mat Engn, Ansan 15588, South Korea
[3] Ajou Univ, Dept Energy Syst Res, Suwon 16499, South Korea
[4] Ajou Univ, Dept Phys, Suwon 16499, South Korea
[5] Korea Basic Sci Inst, Electron Microscopy Res Ctr, Daejeon 169148, South Korea
[6] Chonbuk Natl Univ, IPIT, Jeonju 54896, South Korea
[7] Chonbuk Natl Univ, Dept Phys, Jeonju 54896, South Korea
基金
新加坡国家研究基金会;
关键词
two-dimensional electron gas; atomic layer deposition; field-effect transistor; titanium oxide; aluminum oxide; INTERFACES; ANATASE; SRTIO3;
D O I
10.1021/acsnano.8b05891
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
We report the field-effect transistors using quasi-two-dimensional electron gas generated at an ultrathin (similar to 10 nm) Al2O3/TiO2 heterostructure interface grown via atomic layer deposition (ALD) on a SiO2/Si substrate without using a single crystal substrate. The 2DEG at the Al2O3/TiO2 interface originates from oxygen vacancies generated at the surface of the TiO2 bottom layer during ALD of the Al2O3 overlayer. High-density electrons (similar to 10(14) cm(-2)) are confined within a similar to 2.2 nm distance from the Al2O3/TiO2 interface, resulting in a high on-current of similar to 12 mu A/mu m. The ultrathin TiO2 bottom layer is easy to fully deplete, allowing an extremely low off-current, a high on/off current ratio over 10(8), and a low subthreshold swing of similar to 100 mV/decade. Via the implementation of ALD, a mature thin-film process can facilitate mass production as well as three-dimensional integration of the devices.
引用
收藏
页码:10403 / 10409
页数:7
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