Highly efficient removal of three red dyes by adsorption onto Mg-Al-layered double hydroxide

被引:148
作者
Shan, Ran-ran [1 ]
Yan, Liang-guo [1 ]
Yang, Yan-ming [2 ]
Yang, Kun [1 ]
Yu, Shu-jun [1 ]
Yu, Hai-qin [1 ]
Zhu, Bao-cun [1 ]
Du, Bin [1 ]
机构
[1] Univ Jinan, Sch Resources & Environm, Jinan 250022, Peoples R China
[2] Shandong Cadre Inst Sci & Technol, Jinan 250014, Peoples R China
基金
中国国家自然科学基金;
关键词
Adsorption kinetics; Adsorption isotherm; Reactive red; Congo red; Acid red 1; AQUEOUS-SOLUTION; CONGO-RED; WASTE-WATER; ORANGE; COPRECIPITATION;
D O I
10.1016/j.jiec.2014.03.019
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
The Mg-Al-CO3-LDH with Mg2+/Al3+ molar ratio of 2 was prepared via coprecipitation method at constant pH of 9-10 and used to remove three red dyes by batch adsorption method. The results showed the Mg-Al-LDH were well crystallized and can adsorb the red dyes effectively. The optimal adsorbent dosage and contact time were 1.0 g and 60 min, respectively. Adsorbed amount hardly changed when pH < 10. The adsorption kinetics fit the pseudo-second order kinetic models well and isotherms correspond to Langmuir model strictly. All the relevant mechanisms were studied and manifested as anion exchange and also electrostatic attraction for CR. (C) 2014 The Korean Society of Industrial and Engineering Chemistry. Published by Elsevier B.V. All rights reserved.
引用
收藏
页码:561 / 568
页数:8
相关论文
共 32 条
[21]   Removal of Acid Green 68:1 from aqueous solutions by calcined and uncalcined layered double hydroxides [J].
Menezes dos Santos, Rodrigo Morais ;
Lima Goncalves, Rosembergue Gabriel ;
Leopoldo Constantino, Vera Regina ;
da Costa, Liovando Marciano ;
Mendes da Silva, Luis Henrique ;
Tronto, Jairo ;
Pinto, Frederico Garcia .
APPLIED CLAY SCIENCE, 2013, 80-81 :189-195
[22]   Adsorption and photodegradation properties of anionic dyes by layered double hydroxides [J].
Morimoto, Kazuya ;
Tamura, Kenji ;
Iyi, Nobuo ;
Ye, Jinhua ;
Yamada, Hirohisa .
JOURNAL OF PHYSICS AND CHEMISTRY OF SOLIDS, 2011, 72 (09) :1037-1045
[23]   An investigation on the adsorption of acid dyes on bentonite based composite adsorbent [J].
Qiao, Shizhang ;
Hu, Qiuhong ;
Haghseresht, Fouad ;
Hu, Xijun ;
Lua, Gao Qing .
SEPARATION AND PURIFICATION TECHNOLOGY, 2009, 67 (02) :218-225
[24]   Nickel-iron layered double hydroxide (LDH): Textural properties upon hydrothermal treatments and application on dye sorption [J].
Saiah, Fatiha Boukraa Djellal ;
Su, Bao-Lian ;
Bettahar, Nourredine .
JOURNAL OF HAZARDOUS MATERIALS, 2009, 165 (1-3) :206-217
[25]   Treatment of waters and wastewaters containing sulfur dyes: A review [J].
Thai Anh Nguyen ;
Juang, Ruey-Shin .
CHEMICAL ENGINEERING JOURNAL, 2013, 219 :109-117
[26]   Incorporation of transition metals into Mg-Al layered double hydroxides: Coprecipitation of cations vs. their pre-complexation with an anionic chelator [J].
Tsyganok, Andrey ;
Sayari, Abdelhamid .
JOURNAL OF SOLID STATE CHEMISTRY, 2006, 179 (06) :1830-1841
[27]   Adsorption of As(V) from water using Mg-Fe-based hydrotalcite (FeHT) [J].
Turk, T. ;
Alp, I. ;
Deveci, H. .
JOURNAL OF HAZARDOUS MATERIALS, 2009, 171 (1-3) :665-670
[28]   Phosphate-intercalated Ca-Fe-layered double hydroxides: Crystal structure, bonding character, and release kinetics of phosphate [J].
Woo, Myong A. ;
Kim, Tae Woo ;
Paek, Mi-Jeong ;
Ha, Hyung-Wook ;
Choy, Jin-Ho ;
Hwang, Seong-Ju .
JOURNAL OF SOLID STATE CHEMISTRY, 2011, 184 (01) :171-176
[29]   Coexistence of adsorption and coagulation processes of both arsenate and NOM from contaminated groundwater by nanocrystallined Mg/Al layered double hydroxides [J].
Wu, Xilin ;
Tan, Xiaoli ;
Yang, Shitong ;
Wen, Tao ;
Guo, Hongli ;
Wang, Xiangke ;
Xu, Anwu .
WATER RESEARCH, 2013, 47 (12) :4159-4168
[30]   Adsorption of tripolyphosphate from aqueous solution by Mg-Al-CO3-layered double hydroxides [J].
Xing, Kun ;
Wang, Haizeng ;
Guo, Lugang ;
Song, Weide ;
Zhao, Zhengpeng .
COLLOIDS AND SURFACES A-PHYSICOCHEMICAL AND ENGINEERING ASPECTS, 2008, 328 (1-3) :15-20