Isolated Ni Atoms Dispersed on Ru Nanosheets: High-Performance Electrocatalysts toward Hydrogen Oxidation Reaction

被引:221
作者
Mao, Junjie [1 ]
He, Chun-Ting [2 ]
Pei, Jiajing [3 ]
Liu, Yan [1 ]
Li, Jun [1 ]
Chen, Wenxing [3 ]
He, Dongsheng [4 ]
Wang, Dingsheng [3 ]
Li, Yadong [3 ]
机构
[1] Anhui Normal Univ, Key Lab Electrochem Clean Energy Anhui Higher Edu, Anhui Key Lab Mol Based Mat, Minist Educ,Coll Chem & Mat Sci,Key Lab Funct Mol, Wuhu 241002, Peoples R China
[2] Jiangxi Normal Univ, Key Lab Funct Small Organ Mol, Minist Educ, Coll Chem & Chem Engn, Nanchang, Jiangxi, Peoples R China
[3] Tsinghua Univ, Dept Chem, Beijing 100084, Peoples R China
[4] South Univ Sci & Technol China, Mat Characterizat & Preparat Ctr MCPC, Shenzhen 518055, Guangdong, Peoples R China
基金
中国国家自然科学基金;
关键词
Atomically dispersed; Ru nanocrystals; electrocatalysis; hydrogen oxidation reaction; ALLOY ELECTROCATALYSTS; ALKALINE ELECTROLYTES; NANOPARTICLES; PLATINUM; EVOLUTION; CATALYSTS; SHELL; ELECTROCHEMISTRY; SURFACES; KINETICS;
D O I
10.1021/acs.nanolett.0c00364
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Designing low-cost, high-efficiency, platinum-free electrocatalysts for the hydrogen oxidation reaction (HOR) in an alkaline electrolyte is of great importance for the development of anion exchange membrane fuel cells. Herein, we report a novel HOR catalyst, RuNi1, in which Ni is atomically dispersed on the Ru nanocrystals. To note, the as-prepared RuNi1 catalyst exhibits excellent catalytic activity and stability for HOR in alkaline media, which is superior to those of Ru-Ni bimetallic nanocrystals, pristine Ru, and commercial Pt/C catalysts. Density functional theory (DFT) calculations suggest that isolation of Ni atoms on Ru nanocrystals not only optimizes the hydrogen-binding energy but also decreases the free energy of water formation, thus leading to excellent electrocatalytic activity of RuNi1 catalyst. The results show that engineering a catalyst at an atomic level is highly effective for rational design of electrocatalysts with high performance.
引用
收藏
页码:3442 / 3448
页数:7
相关论文
共 41 条
[1]   Platinum-Coated Copper Nanowires with High Activity for Hydrogen Oxidation Reaction in Base [J].
Alia, Shaun M. ;
Pivovar, Bryan S. ;
Yan, Yushan .
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2013, 135 (36) :13473-13478
[2]   The Effect of Noncovalent Interactions on the HOR, ORR, and HER on Ru, Ir, and Ru0.50Ir0.50 Metal Surfaces in Alkaline Environments [J].
Danilovic, N. ;
Subbaraman, Ram ;
Strmcnik, D. ;
Paulikas, A. P. ;
Myers, D. ;
Stamenkovic, V. R. ;
Markovic, N. M. .
ELECTROCATALYSIS, 2012, 3 (3-4) :221-229
[3]   Golden single-atomic-site platinum electrocatalysts [J].
Duchesne, Paul N. ;
Li, Z. Y. ;
Deming, Christopher P. ;
Fung, Victor ;
Zhao, Xiaojing ;
Yuan, Jun ;
Regier, Tom ;
Aldalbahi, Ali ;
Almarhoon, Zainab ;
Chen, Shaowei ;
Jiang, De-en ;
Zheng, Nanfeng ;
Zhang, Peng .
NATURE MATERIALS, 2018, 17 (11) :1033-+
[4]   Elucidating Hydrogen Oxidation/Evolution Kinetics in Base and Acid by Enhanced Activities at the Optimized Pt Shell Thickness on the Ru Core [J].
Elbert, Katherine ;
Hu, Jue ;
Ma, Zhong ;
Zhang, Yu ;
Chen, Guangyu ;
An, Wei ;
Liu, Ping ;
Isaacs, Hugh S. ;
Adzic, Radoslav R. ;
Wang, Jia X. .
ACS CATALYSIS, 2015, 5 (11) :6764-6772
[5]   Selective catalysts for the hydrogen oxidation and oxygen reduction reactions by patterning of platinum with calix[4]arene molecules [J].
Genorio, Bostjan ;
Strmcnik, Dusan ;
Subbaraman, Ram ;
Tripkovic, Dusan ;
Karapetrov, Goran ;
Stamenkovic, Vojislav R. ;
Pejovnik, Stane ;
Markovic, Nenad M. .
NATURE MATERIALS, 2010, 9 (12) :998-1003
[6]   The road from animal electricity to green energy: combining experiment and theory in electrocatalysis [J].
Greeley, Jeffrey ;
Markovic, Nenad M. .
ENERGY & ENVIRONMENTAL SCIENCE, 2012, 5 (11) :9246-9256
[7]   Robust Phase Control through Hetero-Seeded Epitaxial Growth for Face-Centered Cubic Pt@Ru Nanotetrahedrons with Superior Hydrogen Electro-Oxidation Activity [J].
Gu, Jun ;
Guo, Yu ;
Jiang, Ying-Ying ;
Zhu, Wei ;
Xu, Yan-Shuang ;
Zhao, Ze-Qiong ;
Liu, Jin-Xun ;
Li, Wei-Xue ;
Jin, Chuan-Hong ;
Yan, Chun-Hua ;
Zhang, Ya-Wen .
JOURNAL OF PHYSICAL CHEMISTRY C, 2015, 119 (31) :17697-17706
[8]   Single platinum atoms embedded in nanoporous cobalt selenide as electrocatalyst for accelerating hydrogen evolution reaction [J].
Jiang, Kang ;
Liu, Boyang ;
Luo, Min ;
Ning, Shoucong ;
Peng, Ming ;
Zhao, Yang ;
Lu, Ying-Rui ;
Chan, Ting-Shan ;
de Groot, Frank M. F. ;
Tan, Yongwen .
NATURE COMMUNICATIONS, 2019, 10 (1)
[9]   Transition-Metal Single Atoms in a Graphene Shell as Active Centers for Highly Efficient Artificial Photosynthesis [J].
Jiang, Kun ;
Siahrostami, Samira ;
Akey, Austin J. ;
Li, Yanbin ;
Lu, Zhiyi ;
Lattimer, Judith ;
Hu, Yongfeng ;
Stokes, Chris ;
Gangishetty, Mahesh ;
Chen, Guangxu ;
Zhou, Yawei ;
Hill, Winfield ;
Cai, Wen-Bin ;
Bell, David ;
Chan, Karen ;
Norskov, Jens K. ;
Cui, Yi ;
Wang, Haotian .
CHEM, 2017, 3 (06) :950-960
[10]   Role of Nanomorphology and Interfacial Structure of Platinum Nanoparticles in Catalyzing the Hydrogen Oxidation Reaction [J].
Jiao, Xue ;
Batchelor-McAuley, Christopher ;
Lin, Chuhong ;
Katelhon, Enno ;
Tanner, Eden E. L. ;
Young, Neil P. ;
Compton, Richard G. .
ACS CATALYSIS, 2018, 8 (07) :6192-6202