Enhanced lubricity and anti-wear performance of zwitterionic polymer-modified N-enriched porous carbon nanosheets as water-based lubricant additive

被引:58
作者
Lu, Qi [1 ]
Zhang, Tingting [1 ]
He, Baoluo [1 ]
Xu, Fei [1 ]
Liu, Shujuan [1 ]
Ye, Qian [1 ]
Zhou, Feng [1 ,2 ]
机构
[1] Northwestern Polytech Univ, Ctr Adv Lubricat & Seal Mat, Sch Mat Sci & Engn, State Key Lab Solidificat Proc, Xian 710072, Peoples R China
[2] Chinese Acad Sci, Lanzhou Inst Chem Phys, State Key Lab Solid Lubricat, Lanzhou 730000, Peoples R China
关键词
Water-based lubricant additives; Zwitterion polymer; Porous carbon nanosheets; Friction reduction; TRIBOLOGICAL PERFORMANCE; FRICTION; DOTS; NANOPARTICLES; MECHANISM; GRAPHENE;
D O I
10.1016/j.triboint.2021.107421
中图分类号
TH [机械、仪表工业];
学科分类号
0802 ;
摘要
The zwitterion polymer functionalized N-enriched porous carbon nanosheets were prepared via pyrolysis and etching of pyridine-coordinated polymer for N@PCNS. Subsequently, N@PCNS was modified with polydopamine to grow the zwitterionic polymer (PEIS), thereby acquiring PEIS functionalized N@PCNS (PEIS-PCNS). The exceptional tribological performance of PEIS-PCNS was attributed to the synergistic lubrication effects of N@PCNS along with the zwitterionic polymer PEIS, which facilitates the formation of a stable protective carbon film over the worn surface via complicated tribo-chemical reaction. Meanwhile, the presence of a hydration layer encapsulated by PEIS as the boundary lubricating film proves highly conducive for friction reduction. The average coefficient of friction showed a dramatic decrease to 0.17 from 0.63, and the wear depth of stainless steel dropped 64%.
引用
收藏
页数:10
相关论文
共 44 条
[1]   Hydrophilic nitrogen-doped carbon dots from biowaste using dwarf banana peel for environmental and biological applications [J].
Atchudan, Raji ;
Edison, Thomas Nesakumar Jebakumar Immanuel ;
Perumal, Suguna ;
Muthuchamy, Nallal ;
Lee, Yong Rok .
FUEL, 2020, 275
[2]   Dispersion Stability and Lubrication Mechanism of Nanolubricants [J].
Azman, Nurul Farhanah ;
Samion, Syahrullail .
INTERNATIONAL JOURNAL OF PRECISION ENGINEERING AND MANUFACTURING-GREEN TECHNOLOGY, 2019, 6 (02) :393-414
[3]   Hydroxyapatite supported N-doped carbon quantum dots for visible-light photocatalysis [J].
Chang, Q. ;
Li, K. K. ;
Hu, S. L. ;
Dong, Y. G. ;
Yang, J. L. .
MATERIALS LETTERS, 2016, 175 :44-47
[4]   Ultrastable Lubricating Properties of Robust Self-Repairing Tribofilms Enabled by in Situ-Assembled Polydopamine Nanoparticles [J].
Chen, Guangyan ;
Zhao, Jun ;
Chen, Kai ;
Liu, Siyu ;
Zhang, Minyi ;
He, Yongyong ;
Luo, Jianbin .
LANGMUIR, 2020, 36 (04) :852-861
[5]   Friction and Wear Mechanism of Unlubricated 304L Austenitic Stainless Steel at Room Temperature [J].
Chen Guoqing ;
Wei Yanhui ;
Li Shan ;
Zhou Wenlong .
JOURNAL OF WUHAN UNIVERSITY OF TECHNOLOGY-MATERIALS SCIENCE EDITION, 2012, 27 (02) :222-226
[6]   Polyzwitterionic brushes: Extreme lubrication by design [J].
Chen, Meng ;
Briscoe, Wuge H. ;
Armes, Steven P. ;
Cohen, Hagai ;
Klein, Jacob .
EUROPEAN POLYMER JOURNAL, 2011, 47 (04) :511-523
[7]   Thin films of fullerene-like MoS2 nanoparticles with ultra-low friction and wear [J].
Chhowalla, M ;
Amaratunga, GAJ .
NATURE, 2000, 407 (6801) :164-167
[8]   Graphene-Based Aqueous Lubricants: Dispersion Stability to the Enhancement of Tribological Properties [J].
Chouhan, Ajay ;
Kumari, Sangita ;
Sarkar, Tarun K. ;
Rawat, Sooraj S. ;
Khatri, Om P. .
ACS APPLIED MATERIALS & INTERFACES, 2020, 12 (46) :51785-51796
[9]   Role of nanoparticle materials as water-based lubricant additives for ceramics [J].
Cui, Yuxiao ;
Ding, Mei ;
Sui, Tianyi ;
Zheng, Wei ;
Qiao, Guochao ;
Yan, Shuai ;
Liu, Xibei .
TRIBOLOGY INTERNATIONAL, 2020, 142
[10]   New complexes of heavy lanthanides with 4,4′-bipyridine and trichloroacetates [J].
Czylkowska, A. .
JOURNAL OF THERMAL ANALYSIS AND CALORIMETRY, 2012, 110 (03) :1299-1308