New particle formation under the influence of the long-range transport of air pollutants in East Asia

被引:18
作者
Chandra, Indra [1 ]
Kim, Seyoung [1 ]
Seto, Takafumi [1 ]
Otani, Yoshio [1 ]
Takami, Akinori [2 ]
Yoshino, Ayako [2 ]
Irei, Satoshi [2 ]
Park, Kihong [3 ]
Takamura, Tamio [4 ]
Kaneyasu, Naoki [5 ]
Hatakeyama, Shiro [6 ]
机构
[1] Kanazawa Univ, Dept Chem & Mat Engn, Kanazawa, Ishikawa 9201192, Japan
[2] Natl Inst Environm Studies, Ctr Reg Environm Res, 16-2 Onogawa, Tsukuba, Ibaraki 3058506, Japan
[3] Gwangju Inst Sci & Technol, Sch Environm Sci & Engn, 261 Cheomdan Gwagiro, Gwangju 500712, South Korea
[4] Chiba Univ, Ctr Environm Remote Sensing CEReS, Chiba 2638522, Japan
[5] Natl Inst Adv Ind Sci & Technol, Global Environm Study Grp, 16-1 Onogawa, Tsukuba, Ibaraki 3058568, Japan
[6] Tokyo Univ Agr & Technol, Inst Agr, 3-5-8 Saiwaicho, Fuchu, Tokyo 1838509, Japan
关键词
New particle formation; Aerosol; Long-range transport; East Asia; NUCLEATION MODE PARTICLES; NUMBER SIZE DISTRIBUTIONS; NORTH CHINA PLAIN; ATMOSPHERIC NUCLEATION; FORMATION EVENTS; BOUNDARY-LAYER; GROWTH EVENTS; SULFURIC-ACID; FUKUE ISLAND; RURAL SITES;
D O I
10.1016/j.atmosenv.2016.06.040
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Field observations to investigate the correlation between New Particle Formation (NPF) and the long-range transport of air pollutants in the East Asia region were carried out on a rural Island of Japan in the East-China Sea (Fukue Island, 32.8 degrees N, 128.7 degrees E) over three periods (February 23 to March 7, 2013; November 7 to 20, 2013; and November 2 to 24, 2014). Frequent NPF events were identified (16 events in 50 days), typically in association with sudden increases in particle number concentrations and the successive growth of particles to mobility diameters of several tens of nanometers. The NPF events were classified into two types (A and B) according to the initially detected particle sizes (onset diameters). Type-A consisted of strong NPF events with onset diameters as small as 5 nm. Type-B consisted of NPF events whose onset (<10 nm) was not clearly identifiable. The correlations of SO2 concentrations, solar radiation, PM2.5 concentrations, and chemical composition were analyzed based on the types of NPF events. (C) 2016 Elsevier Ltd. All rights reserved.
引用
收藏
页码:30 / 40
页数:11
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