Spray-cast multilayer perovskite solar cells with an active-area of 1.5 cm2

被引：69
|
作者：
Bishop, James E. [1 ]
Mohamad, David K. [1 ]
Wong-Stringer, Michael [1 ]
Smith, Alex [2 ]
Lidzey, David G. [1 ]
机构：
[1] Univ Sheffield, Dept Phys & Astron, Hicks Bldg,Hounsfield Rd, Sheffield S3 7RH, S Yorkshire, England
[2] Loughborough Univ, Wolfson Sch, CREST, Loughborough LE11 3TU, Leics, England
来源：
SCIENTIFIC REPORTS | 2017年 / 7卷
基金：
英国工程与自然科学研究理事会;
关键词：
HIGH-PERFORMANCE; HALIDE PEROVSKITE; THIN-FILM; EFFICIENT; PHOTOVOLTAICS; FABRICATION; DEPOSITION; TRIHALIDE; PHOTORESIST; CONVERSION;
D O I：
10.1038/s41598-017-08642-2
中图分类号：
O [数理科学和化学]; P [天文学、地球科学]; Q [生物科学]; N [自然科学总论];
学科分类号：
07 ; 0710 ; 09 ;
摘要：
We utilise spray-coating under ambient conditions to sequentially deposit compact-TiO2, mesoporous-TiO2, CH3NH3PbI(3-x) Cl-x perovskite and doped spiro-OMeTAD layers, creating a mesoporous standard architecture perovskite solar cell (PSC). The devices created had an average power conversion efficiency (PCE) of 9.2% and a peak PCE of 10.2%; values that compare favourably with control-devices fabricated by spin-casting that had an average efficiency of 11.4%. We show that our process can be used to create devices having an active-area of 1.5 cm(2) having an independently verified efficiency of 6.6%. This work demonstrates the versatility of spray-coating as well as its potential as a method of manufacturing lowcost, large-area, efficient perovskite devices.
引用
收藏
页数：11
相关论文
共 50 条
  • [21] Stable and sustainable perovskite solar modules by optimizing blade coating nickel oxide deposition over 15 x 15 cm2 area
    Jafarzadeh, Farshad
    Castriotta, Luigi Angelo
    Calabro, Emanuele
    Spinelli, Pierpaolo
    Generosi, Amanda
    Paci, Barbara
    Rodriguez, David Becerril
    Luce, Marco
    Cricenti, Antonio
    Di Giacomo, Francesco
    Matteocci, Fabio
    Brunetti, Francesca
    Di Carlo, Aldo
    COMMUNICATIONS MATERIALS, 2024, 5 (01)
  • [22] Comparison of Physical Isolation on Large Active Area Perovskite Solar Cells
    Gao, Liguo
    Yan, Yeling
    Li, Yang
    Ma, Tingli
    CHEMICAL RESEARCH IN CHINESE UNIVERSITIES, 2020, 36 (06) : 1279 - 1283
  • [23] Perovskite/Silicon Tandem Solar Cells with a Voc of 1784 mV Based on an Industrially Feasible 25 cm2 TOPCon Silicon Cell
    Hyun, Ji Yeon
    Yeom, Kyung Mun
    Lee, Sang-Won
    Bae, Soohyun
    Choi, Dongjin
    Song, Hoyoung
    Kang, Dongkyun
    Hwang, Jae-Keun
    Lee, Wonkyu
    Lee, Solhee
    Kang, Yoonmook
    Lee, Hae-Seok
    Noh, Jun Hong
    Kim, Donghwan
    ACS APPLIED ENERGY MATERIALS, 2022, 5 (05): : 5449 - 5456
  • [24] Bio-Inspired Graphitic Carbon-Based Large-Area (10 x 10 cm2) Perovskite Solar Cells: Stability Assessments under Indoor, Outdoor, and Water-Soaked Conditions
    Pitchaiya, Selvakumar
    Eswaramoorthy, Nandhakumar
    Ramakrishnan, Venkatraman Madurai
    Natarajan, Muthukumarasamy
    Velauthapillai, Dhayalan
    ACS APPLIED MATERIALS & INTERFACES, 2022, 14 (38) : 43050 - 43066
  • [25] Highly stable perovskite solar cells based on perovskite/NiO-graphene composites and NiO interface with 25.9 mA/cm2 photocurrent density and 20.8% efficiency
    Mahmoudi, Tahmineh
    Wang, Yousheng
    Hahn, Yoon-Bong
    NANO ENERGY, 2021, 79 (79)
  • [26] 21.8% Efficient Monolithic Perovskite/Homo-Junction-Silicon Tandem Solar Cell on 16 cm2
    Zheng, Jianghui
    Mehrvarz, Hamid
    Ma, Fa-Jun
    Lau, Cho Fai Jonathan
    Green, Martin A.
    Huang, Shujuan
    Ho-Baillie, Anita W. Y.
    ACS ENERGY LETTERS, 2018, 3 (09): : 2299 - 2300
  • [27] 54 cm2 Large-Area Flexible Organic Solar Modules with Efficiency Above 13%
    Qin, Fei
    Sun, Lulu
    Chen, Hongting
    Liu, Yang
    Lu, Xin
    Wang, Wen
    Liu, Tiefeng
    Dong, Xinyun
    Jiang, Pei
    Jiang, Youyu
    Wang, Lei
    Zhou, Yinhua
    ADVANCED MATERIALS, 2021, 33 (39)
  • [28] Decoupled Water Electrolysis Driven by 1 cm2 Single Perovskite Solar Cell Yielding a Solar-to-Hydrogen Efficiency of 14.4 %
    Lv, Fei
    Qin, Zhixiao
    Wu, Jiazhe
    Pan, Lixia
    Liu, Longjie
    Chen, Yubin
    Zhao, Yixin
    CHEMSUSCHEM, 2022, 16 (01)
  • [29] Reticulated Mesoporous TiO2 Scaffold, Fabricated by Spray Coating, for Large-Area Perovskite Solar Cells
    Tomulescu, Andrei Gabriel
    Stancu, Viorica
    Besleaga, Cristina
    Enculescu, Monica
    Nemnes, George Alexandru
    Florea, Mihaela
    Dumitru, Viorel
    Pintilie, Lucian
    Pintilie, Ioana
    Leonat, Lucia
    ENERGY TECHNOLOGY, 2020, 8 (01)
  • [30] Natural Amino Acid Enables Scalable Fabrication of High-Performance Flexible Perovskite Solar Cells and Modules with Areas over 300 cm2
    Wu, Ziyi
    Liu, Xuanling
    Zhong, Han
    Wu, Zhihao
    Chen, Hao
    Su, Jiazheng
    Xu, Youcheng
    Wang, Xuanyu
    Li, Xin
    Lin, Hong
    SMALL METHODS, 2022, 6 (12)
12345