Atmospheric Aerosols: Clouds, Chemistry, and Climate

被引:99
作者
McNeill, V. Faye [1 ]
机构
[1] Columbia Univ, Dept Chem Engn, New York, NY 10027 USA
来源
ANNUAL REVIEW OF CHEMICAL AND BIOMOLECULAR ENGINEERING, VOL 8 | 2017年 / 8卷
基金
美国国家科学基金会;
关键词
air quality; atmospheric chemistry; chemical engineering; environment; geoengineering; CHARGE-TRANSFER COMPLEXES; BROWN CARBON; OPTICAL-PROPERTIES; MASS-SPECTROMETER; ORGANIC-COMPOUNDS; AQUEOUS AEROSOL; HUMIC-LIKE; PARTICLE NUCLEATION; URBAN-ENVIRONMENT; AMBIENT AEROSOLS;
D O I
10.1146/annurev-chembioeng-060816-101538
中图分类号
O69 [应用化学];
学科分类号
081704 ;
摘要
Although too small to be seen with the human eye, atmospheric particulate matter has major impacts on the world around us, from our health to global climate. Understanding the sources, properties, and transformations of these particles in the atmosphere is among the major challenges in air quality and climate research today. Significant progress has been made over the past two decades in understanding atmospheric aerosol chemistry and its connections to climate. Advances in technology for characterizing aerosol chemical composition and physical properties have enabled rapid discovery in this area. This article reviews fundamental concepts and recent developments surrounding ambient aerosols, their chemical composition and sources, light-absorbing aerosols, aerosols and cloud formation, and aerosol-based solar radiation management (also known as solar geoengineering).
引用
收藏
页码:427 / 444
页数:18
相关论文
共 165 条
[1]   Solid ammonium sulfate aerosols as ice nuclei:: A pathway for cirrus cloud formation [J].
Abbatt, J. P. D. ;
Benz, S. ;
Cziczo, D. J. ;
Kanji, Z. ;
Lohmann, U. ;
Moehler, O. .
SCIENCE, 2006, 313 (5794) :1770-1773
[2]   Resolving anthropogenic aerosol pollution types - deconvolution and exploratory classification of pollution events [J].
Aijala, Mikko ;
Heikkinen, Liine ;
Frohlich, Roman ;
Canonaco, Francesco ;
Prevot, Andre S. H. ;
Junninen, Heikki ;
Petaja, Tuukka ;
Kulmala, Markku ;
Worsnop, Douglas ;
Ehn, Mikael .
ATMOSPHERIC CHEMISTRY AND PHYSICS, 2017, 17 (04) :3165-3197
[3]   Cytotoxic and proinflammatory effects of ambient and source-related particulate matter (PM) in relation to the production of reactive oxygen species (ROS) and cytokine adsorption by particles [J].
Akhtar, Umme S. ;
McWhinney, Robert D. ;
Rastogi, Neeraj ;
Abbatt, Jonathan P. D. ;
Evans, Greg J. ;
Scott, Jeremy A. .
INHALATION TOXICOLOGY, 2010, 22 :37-47
[4]   AEROSOLS, CLOUD MICROPHYSICS, AND FRACTIONAL CLOUDINESS [J].
ALBRECHT, BA .
SCIENCE, 1989, 245 (4923) :1227-1230
[5]   Reversal of ocean acidification enhances net coral reef calcification [J].
Albright, Rebecca ;
Caldeira, Lilian ;
Hosfelt, Jessica ;
Kwiatkowski, Lester ;
Maclaren, Jana K. ;
Mason, Benjamin M. ;
Nebuchina, Yana ;
Ninokawa, Aaron ;
Pongratz, Julia ;
Ricke, Katharine L. ;
Rivlin, Tanya ;
Schneider, Kenneth ;
Sesbouee, Marine ;
Shamberger, Kathryn ;
Silverman, Jacob ;
Wolfe, Kennedy ;
Zhu, Kai ;
Caldeira, Ken .
NATURE, 2016, 531 (7594) :362-+
[6]   Brown carbon spheres in East Asian outflow and their optical properties [J].
Alexander, Duncan T. L. ;
Crozier, Peter A. ;
Anderson, James R. .
SCIENCE, 2008, 321 (5890) :833-836
[7]   Molecular understanding of sulphuric acid-amine particle nucleation in the atmosphere [J].
Almeida, Joao ;
Schobesberger, Siegfried ;
Kuerten, Andreas ;
Ortega, Ismael K. ;
Kupiainen-Maatta, Oona ;
Praplan, Arnaud P. ;
Adamov, Alexey ;
Amorim, Antonio ;
Bianchi, Federico ;
Breitenlechner, Martin ;
David, Andre ;
Dommen, Josef ;
Donahue, Neil M. ;
Downard, Andrew ;
Dunne, Eimear ;
Duplissy, Jonathan ;
Ehrhart, Sebastian ;
Flagan, Richard C. ;
Franchin, Alessandro ;
Guida, Roberto ;
Hakala, Jani ;
Hansel, Armin ;
Heinritzi, Martin ;
Henschel, Henning ;
Jokinen, Tuija ;
Junninen, Heikki ;
Kajos, Maija ;
Kangasluoma, Juha ;
Keskinen, Helmi ;
Kupc, Agnieszka ;
Kurten, Theo ;
Kvashin, Alexander N. ;
Laaksonen, Ari ;
Lehtipalo, Katrianne ;
Leiminger, Markus ;
Leppa, Johannes ;
Loukonen, Ville ;
Makhmutov, Vladimir ;
Mathot, Serge ;
McGrath, Matthew J. ;
Nieminen, Tuomo ;
Olenius, Tinja ;
Onnela, Antti ;
Petaja, Tuukka ;
Riccobono, Francesco ;
Riipinen, Ilona ;
Rissanen, Matti ;
Rondo, Linda ;
Ruuskanen, Taina ;
Santos, Filipe D. .
NATURE, 2013, 502 (7471) :359-+
[8]   Black carbon or brown carbon?: The nature of light-absorbing carbonaceous aerosols [J].
Andreae, M. O. ;
Gelencser, A. .
ATMOSPHERIC CHEMISTRY AND PHYSICS, 2006, 6 :3131-3148
[9]  
[Anonymous], FUT ATM CHEM RES
[10]  
[Anonymous], 2014, ARS CLIM CHANG 2014