Electronic Light-Matter Strong Coupling in Nanofluidic Fabry-Perot Cavities

被引：32

作者：

Bahsoun, Hadi ^{[1
,2
]}

Chervy, Thibault ^{[1
,2
]}

Thomas, Anoop ^{[1
,2
]}

Borjesson, Karl ^{[3
]}

Hertzog, Manuel ^{[1
,2
]}

George, Jino ^{[1
,2
]}

Devaux, Eloise ^{[1
,2
]}

Genet, Cyriaque ^{[1
,2
]}

Hutchison, James A. ^{[1
,2
]}

Ebbesen, Thomas W. ^{[1
,2
]}

机构：

[1] Univ Strasbourg, CNRS, ISIS, 8 Allee Gaspard Monge, F-67000 Strasbourg, France

[2] Univ Strasbourg, CNRS, icFRC, 8 Allee Gaspard Monge, F-67000 Strasbourg, France

[3] Univ Gothenburg, Dept Chem & Mol Biol, S-41296 Gothenburg, Sweden

来源：

ACS PHOTONICS | 2018年 / 5卷 / 01期

关键词：

Rabi splitting; Chlorin e6; quantum yield; fluorescence lifetime decay; radiative and nonradiative decay rates; SURFACE-PLASMON POLARITONS; DYNAMICS; PORPHYRIN; MOLECULES; EMISSION; STATES; MODES; WEAK; DYE;

D O I：

10.1021/acsphotonics.7b00679

中图分类号：

TB3 [工程材料学];

学科分类号：

0805 ; 080502 ;

摘要：

Electronic light-matter strong coupling has been limited to solid molecular films due to the challenge of preparing optical cavities with nanoscale dimensions. Here we report a technique to fabricate such Fabry-Perot nanocavities in which solutions can be introduced such that light molecule interactions can be studied at will in the liquid phase. We illustrate the versatility of these cavities by studying the emission properties of Chlorin e6 solutions in both the weak and strong coupling regimes as a function of cavity detuning. Liquid nanocavities will broaden the investigation of strong coupling to many solution-based molecular processes.

引用

页码：225 / 232

页数：8

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