Nitrate reduction in water catalysed by Pd-Cu on different supports

被引：88

作者：

Soares, Olivia Salome G. P. ^{[1
]}

Orfao, Jose J. M. ^{[1
]}

Pereira, Manuel Fernando R. ^{[1
]}

机构：

[1] Univ Porto, Fac Engn, Dept Engn Quim, LCM,Lab Assoc LSRE LCM, P-4200465 Oporto, Portugal

来源：

DESALINATION | 2011年 / 279卷 / 1-3期

关键词：

Nitrate reduction; Metal oxides; Activated carbon; Carbon nanotubes; Pd-Cu; PALLADIUM-BASED CATALYSTS; PT-CU; BIMETALLIC CATALYSTS; ACTIVATED CARBON; SELECTIVE HYDROGENATION; TOTAL OXIDATION; COPPER; REMOVAL; NITRITE; DENITRIFICATION;

D O I：

10.1016/j.desal.2011.06.037

中图分类号：

TQ [化学工业];

学科分类号：

0817 ;

摘要：

Screening tests were carried out in order to study the influence of the support in the performance of Pd monometallic and Pd-Cu bimetallic catalysts for the reduction of nitrate in water. Several metal oxides, as well as metal oxides and activated carbon or carbon nanotube composites were assessed as supports. The catalysts were prepared and tested under the same operation conditions. It was observed that supports play an important role in the catalytic performance and in some cases are directly involved in the reaction mechanism. The Pd-Cu catalysts supported on titanium dioxide and on the composite containing carbon nanotubes and titanium dioxide present the highest conversions, while those supported on ceria materials are the most selective to nitrogen. (C) 2011 Elsevier B.V. All rights reserved.

引用

页码：367 / 374

页数：8

共 50 条

[41] The oxidation state of copper in bimetallic (Pt-Cu, Pd-Cu) catalysts during water denitration [J].

Sa, Jacinto ;

Barrabes, Noelia ;

Kleymenov, Evgeny ;

Lin, Chen ;

Foettinger, Karin ;

Safonova, Olga V. ;

Szlachetko, Jakub ;

van Bokhoven, Jeroen A. ;

Nachtegaal, Maarten ;

Urakawa, Atsushi ;

Crespo, Gaston A. ;

Rupprechter, Guenther .

CATALYSIS SCIENCE & TECHNOLOGY, 2012, 2 (04) :794-799

[42] Diversity of Pd-Cu active sites supported on pristine carbon nanotubes in terms of water denitration structure sensitivity [J].

Panic, Sanja ;

Srdic, Vladimir ;

Varga, Tamas ;

Konya, Zoltan ;

Kukovecz, Akos ;

Boskovic, Goran .

APPLIED CATALYSIS A-GENERAL, 2018, 559 :187-194

[43] Catalytic Hydrogenation of Nitrate Ions over Pd-Cu/ZSM-5 Catalyst [J].

Gao, Wenliang ;

Li, Fang .

NEW AND ADVANCED MATERIALS, PTS 1 AND 2, 2011, 197-198 :967-971

[44] Catalytic reduction of bromate over monometallic catalysts on different powder and structured supports [J].

Restivo, J. ;

Soares, O. S. G. P. ;

Orfao, J. J. M. ;

Pereira, M. F. R. .

CHEMICAL ENGINEERING JOURNAL, 2017, 309 :197-205

[45] Activity and Stability of Pd Bimetallic Catalysts for Catalytic Nitrate Reduction [J].

Sanchis, Ines ;

Jose Rodriguez, Juan ;

Mohedano, Angel F. ;

Diaz, Elena .

CATALYSTS, 2022, 12 (07)

[46] Pd and Pd-Cu supported on different carbon materials and immobilized as flow-through catalytic membranes for the chemical reduction of NO3-, NO-2 and BrO3- in drinking water treatment [J].

Mari, Adrian ;

Baeza, Jose Alberto ;

Pedrosa, Marta ;

Soares, O. Salome G. P. ;

Calvo, Luisa ;

Gilarranz, Miguel Angel ;

Silva, Adrian M. T. ;

Pereira, M. Fernando R. .

JOURNAL OF ENVIRONMENTAL CHEMICAL ENGINEERING, 2023, 11 (03)

[47] Mono and bimetallic NaY catalysts with high performance in nitrate reduction in water [J].

Soares, Olivia S. G. P. ;

Marques, Luisa ;

Freitas, Catia M. A. S. ;

Fonseca, Antonio M. ;

Parpot, Pier ;

Orfao, Jose J. M. ;

Pereira, Manuel F. R. ;

Neves, Isabel C. .

CHEMICAL ENGINEERING JOURNAL, 2015, 281 :411-417

[48] Nitrate reduction by maghemite supported Cu-Pd bimetallic catalyst [J].

Jung, Junyoung ;

Bae, Sungjun ;

Lee, Woojin .

APPLIED CATALYSIS B-ENVIRONMENTAL, 2012, 127 :148-158

[49] Engineering of Nanostructured Carbon Catalyst Supports for the Continuous Reduction of Bromate in Drinking Water [J].

da Costa, Joao M. Cunha Bessa ;

Barbosa, Jose R. Monteiro ;

Restivo, Joao ;

Orge, Carla A. ;

Nogueira, Anabela ;

Castro-Silva, Sergio ;

Pereira, Manuel F. Ribeiro ;

Soares, Olivia S. Goncalves Pinto .

C-JOURNAL OF CARBON RESEARCH, 2022, 8 (02)

[50] Combination of Pd-Cu Catalysis and Electrolytic H2 Evolution for Selective Nitrate Reduction Using Protonated Polypyrrole as a Cathode [J].

Chen, Chen ;

Li, Kan ;

Li, Chen ;

Sun, Tonghua ;

Jia, Jinping .

ENVIRONMENTAL SCIENCE & TECHNOLOGY, 2019, 53 (23) :13868-13877

← 1 2 3 4 5 →