A perylene diimide (PDI)-based small molecule with tetrahedral configuration as a non-fullerene acceptor for organic solar cells

被引：185
作者：
Chen, Wangqiao [1 ,2 ]
Yang, Xuan [3 ]
Long, Guankui [1 ,3 ]
Wan, Xiangjian [3 ]
Chen, Yongsheng [3 ]
Zhang, Qichun [1 ,2 ,4 ]
机构：
[1] Nanyang Technol Univ, Sch Mat Sci & Engn, Singapore 639798, Singapore
[2] Nanyang Technol Univ, Inst Sports Res, Singapore 639798, Singapore
[3] Nankai Univ, Collaborat Ctr Chem Sci & Engn Tianjin, Key Lab Funct Polymer Mat,Coll Chem, Ctr Nanoscale Sci & Technol,Inst Polymer Chem, Tianjin 300071, Peoples R China
[4] Nanyang Technol Univ, Sch Phys & Math Sci, Div Chem & Biol Chem, Singapore 637371, Singapore
来源：
JOURNAL OF MATERIALS CHEMISTRY C | 2015年 / 3卷 / 18期
关键词：
OPEN-CIRCUIT VOLTAGE; FIELD-EFFECT TRANSISTORS; PHOTOPHYSICAL PROPERTIES; NONFULLERENE ACCEPTORS; MICROPOROUS POLYIMIDES; BUILDING-BLOCKS; HIGH-MOBILITY; POLYMER; PERFORMANCE; EFFICIENCY;
D O I：
10.1039/c5tc00865d
中图分类号：
T [工业技术];
学科分类号：
08 ;
摘要：
In this paper, a new perylene diimide (PDI)-based acceptor Me-PDI4 with tetrahedral configuration (or 3D) has been synthesized and characterized. Solution-processed organic solar cells (OSCs) based on Me-PDI4 have been investigated and our results show that the device performance can reach as high as 2.73%. Our new design with tetrahedral configuration (or 3D) could be an efficient approach to increase the PCE of OSCs with non-fullerene acceptors.
引用
收藏
页码：4698 / 4705
页数：8
相关论文
共 89 条
[1]   An electron acceptor based on indacenodithiophene and 1,1-dicyanomethylene-3-indanone for fullerene-free organic solar cells [J].
Bai, Huitao ;
Wang, Yifan ;
Cheng, Pei ;
Wang, Jiayu ;
Wu, Yao ;
Hou, Jianhui ;
Zhan, Xiaowei .
JOURNAL OF MATERIALS CHEMISTRY A, 2015, 3 (05) :1910-1914
[2]   Acceptor Properties of Boron Subphthalocyanines in Fullerene Free Photovoltaics [J].
Beaumont, Nicola ;
Castrucci, Jeffrey S. ;
Sullivan, Paul ;
Morse, Graham E. ;
Paton, Andrew S. ;
Lu, Zheng-Hong ;
Bender, Timothy P. ;
Jones, Tim S. .
JOURNAL OF PHYSICAL CHEMISTRY C, 2014, 118 (27) :14813-14823
[3]   DENSITY-FUNCTIONAL THERMOCHEMISTRY .3. THE ROLE OF EXACT EXCHANGE [J].
BECKE, AD .
JOURNAL OF CHEMICAL PHYSICS, 1993, 98 (07) :5648-5652
[4]   Hybrid zinc oxide conjugated polymer bulk heterojunction solar cells [J].
Beek, WJE ;
Wienk, MM ;
Kemerink, M ;
Yang, XN ;
Janssen, RAJ .
JOURNAL OF PHYSICAL CHEMISTRY B, 2005, 109 (19) :9505-9516
[5]   Single-Junction Polymer Solar Cells Exceeding 10% Power Conversion Efficiency [J].
Chen, Jing-De ;
Cui, Chaohua ;
Li, Yan-Qing ;
Zhou, Lei ;
Ou, Qing-Dong ;
Li, Chi ;
Li, Yongfang ;
Tang, Jian-Xin .
ADVANCED MATERIALS, 2015, 27 (06) :1035-1041
[6]   A new ladder-type benzodi(cyclopentadithiophene)-based donor-acceptor polymer and a modified hole-collecting PEDOT: PSS layer to achieve tandem solar cells with an open-circuit voltage of 1.62 V [J].
Chen, Yung-Lung ;
Kao, Wei-Shun ;
Tsai, Che-En ;
Lai, Yu-Ying ;
Cheng, Yen-Ju ;
Hsu, Chain-Shu .
CHEMICAL COMMUNICATIONS, 2013, 49 (70) :7702-7704
[7]   Binary additives synergistically boost the efficiency of all-polymer solar cells up to 3.45% [J].
Cheng, Pei ;
Ye, Long ;
Zhao, Xingang ;
Hou, Jianhui ;
Li, Yongfang ;
Zhan, Xiaowei .
ENERGY & ENVIRONMENTAL SCIENCE, 2014, 7 (04) :1351-1356
[8]   Synthesis of Conjugated Polymers for Organic Solar Cell Applications [J].
Cheng, Yen-Ju ;
Yang, Sheng-Hsiung ;
Hsu, Chain-Shu .
CHEMICAL REVIEWS, 2009, 109 (11) :5868-5923
[9]   Rational design on n-type organic materials for high performance organic photovoltaics [J].
Chochos, Christos L. ;
Tagmatarchis, Nikos ;
Gregoriou, Vasilis G. .
RSC ADVANCES, 2013, 3 (20) :7160-7181
[10]   Insights from Transient Optoelectronic Analyses on the Open-Circuit Voltage of Organic Solar Cells [J].
Credgington, Dan ;
Durrant, James R. .
JOURNAL OF PHYSICAL CHEMISTRY LETTERS, 2012, 3 (11) :1465-1478
123456789