Trimethyl lock: a trigger for molecular release in chemistry, biology, and pharmacology

被引:114
作者
Levine, Michael N. [1 ]
Raines, Ronald T. [1 ,2 ]
机构
[1] Univ Wisconsin, Dept Biochem, Madison, WI 53706 USA
[2] Univ Wisconsin, Dept Chem, Madison, WI 53706 USA
关键词
HYDROXY AMIDE LACTONIZATION; INTRAMOLECULAR CONJUGATE ADDITION; STEREOPOPULATION-CONTROL; ALKALINE-PHOSPHATASE; PEPTIDE-BOND; DELIVERY SYSTEMS; LATENT FLUOROPHORE; RATE ENHANCEMENT; ANTITUMOR AGENT; AMINE PRODRUGS;
D O I
10.1039/c2sc20536j
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
The trimethyl lock is an o-hydroxydihydrocinnamic acid derivative in which unfavorable steric interactions between three pendant methyl groups encourage lactonization to form a hydrocoumarin. This reaction is extremely rapid, even when the electrophile is an amide and the leaving group is an amino group of a small-molecule drug, fluorophore, peptide, or nucleic acid. O-Acylation of the phenolic hydroxyl group prevents reaction, providing a trigger for the reaction. Thus, the release of an amino group from an amide can be coupled to the hydrolysis of a designated ester (or to another chemical reaction that regenerates the hydroxyl group). Trimethyl lock conjugates are easy to synthesize, making the trimethyl lock a highly versatile module for chemical biology and related fields.
引用
收藏
页码:2412 / 2420
页数:9
相关论文
共 67 条
[1]   AMINE PRODRUGS WHICH UTILIZE HYDROXY AMIDE LACTONIZATION .2. A POTENTIAL ESTERASE-SENSITIVE AMIDE PRODRUG [J].
AMSBERRY, KL ;
GERSTENBERGER, AE ;
BORCHARDT, RT .
PHARMACEUTICAL RESEARCH, 1991, 8 (04) :455-461
[2]   AMINE PRODRUGS WHICH UTILIZE HYDROXY AMIDE LACTONIZATION .1. A POTENTIAL REDOX-SENSITIVE AMIDE PRODRUG [J].
AMSBERRY, KL ;
BORCHARDT, RT .
PHARMACEUTICAL RESEARCH, 1991, 8 (03) :323-330
[3]  
[Anonymous], 2003, HYDROLYSIS DRUG PROD
[4]   Synthesis and applications of Rhodamine derivatives as fluorescent probes [J].
Beija, Mariana ;
Afonso, Carlos A. M. ;
Martinho, Jose M. G. .
CHEMICAL SOCIETY REVIEWS, 2009, 38 (08) :2410-2433
[5]   STEREOPOPULATION CONTROL .3. FACILITATION OF INTRAMOLECULAR CONJUGATE ADDITION OF CARBOXYL GROUP [J].
BORCHARD.RT ;
COHEN, LA .
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 1972, 94 (26) :9175-9182
[6]   STEREOPOPULATION CONTROL .2. RATE ENHANCEMENT OF INTRAMOLECULAR NUCLEOPHILIC DISPLACEMENT [J].
BORCHARD.RT ;
COHEN, LA .
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 1972, 94 (26) :9166-9174
[8]   Direct measurement of the uncatalyzed rate of hydrolysis of a peptide bond [J].
Bryant, RAR ;
Hansen, DE .
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 1996, 118 (23) :5498-5499
[9]   Latent fluorophore based on the trimethyl lock [J].
Chandran, SS ;
Dickson, KA ;
Raines, RT .
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2005, 127 (06) :1652-1653
[10]   Cellular Uptake of Ribonuclease A Relies on Anionic Glycans [J].
Chao, Tzu-Yuan ;
Lavis, Luke D. ;
Raines, Ronald T. .
BIOCHEMISTRY, 2010, 49 (50) :10666-10673