Dinaphthoporphycenes: Synthesis and Nonlinear Optical Studies

被引：104
|
作者：
Sarma, Tridib [1 ]
Panda, Pradeepta K. [1 ,2 ]
Anusha, P. T. [2 ]
Rao, S. Venugopal [2 ]
机构：
[1] Univ Hyderabad, Sch Chem, Hyderabad 500046, Andhra Pradesh, India
[2] Univ Hyderabad, ACRHEM, Hyderabad 500046, Andhra Pradesh, India
来源：
ORGANIC LETTERS | 2011年 / 13卷 / 02期
关键词：
2-PHOTON ABSORPTION; 3-PHOTON ABSORPTION; PORPHYCENE; PORPHYRINS; PYRROLOINDOLES; COMPLEXES; MOLECULES; HYDROGEN;
D O I：
10.1021/ol102378g
中图分类号：
O62 [有机化学];
学科分类号：
070303 ; 081704 ;
摘要：
Naphthobipyrrole-derived porphycenes are synthesized for the first time via McMurry coupling of the beta-alkylated 2,9-diformylnaphthobipyrrole derivatives, which in turn were prepared easily from 2,3-naphthalene bishydrazine in four steps. Insertion of nickel into the porphycene core results in transformation of the rectangular N4-core into a square type geometry owing to the fusion of naphthalene moiety onto the bipyrrole entities. These porphycenes show large, intensity dependent three-photon absorption.
引用
收藏
页码：188 / 191
页数：4
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