Increases in aerosol concentrations over eastern China due to the decadal-scale weakening of the East Asian summer monsoon

被引:161
|
作者
Zhu, Jianlei [1 ,2 ,3 ]
Liao, Hong [1 ]
Li, Jianping [2 ]
机构
[1] Chinese Acad Sci, Inst Atmospher Phys, State Key Lab Atmospher Boundary Layer Phys & Atm, Beijing 100029, Peoples R China
[2] Chinese Acad Sci, Inst Atmospher Phys, State Key Lab Numer Modeling Atmospher Sci & Geop, Beijing 100029, Peoples R China
[3] Chinese Acad Sci, Grad Univ, Beijing 100029, Peoples R China
基金
中国国家自然科学基金;
关键词
SPATIAL-DISTRIBUTION; UNITED-STATES; PART I; CLIMATE; PM2.5; SULFATE; VISIBILITY; INVENTORY; EMISSIONS; TRANSPORT;
D O I
10.1029/2012GL051428
中图分类号
P [天文学、地球科学];
学科分类号
07 ;
摘要
China has been experiencing increased concentrations of aerosols, commonly attributed to the large increases in emissions associated with the rapid economic development. We show by using a chemical transport model driven by the assimilated meteorological fields that the observed decadal-scale weakening of the East Asian summer monsoon also contributed to the increases in aerosols in China. We find that the simulated aerosol concentrations have strong negative correlations with the strength of the East Asian Summer monsoon. Accounting for sulfate, nitrate, ammonium, black carbon, and organic carbon aerosols, the summer surface-layer PM2.5 concentration averaged over eastern China (110 degrees-125 degrees E, 20 degrees-45 degrees N) can be 17.7% higher in the weakest monsoon years than in the strongest monsoon years. The weakening of the East Asian Summer monsoon increases aerosol concentrations mainly by the changes in atmospheric circulation (the convergence of air pollutants) in eastern China. Citation: Zhu, J., H. Liao, and J. Li (2012), Increases in aerosol concentrations over eastern China due to the decadal-scale weakening of the East Asian summer monsoon, Geophys. Res. Lett., 39, L09809, doi: 10.1029/2012GL051428.
引用
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页数:6
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