Increases in aerosol concentrations over eastern China due to the decadal-scale weakening of the East Asian summer monsoon

被引:161
作者
Zhu, Jianlei [1 ,2 ,3 ]
Liao, Hong [1 ]
Li, Jianping [2 ]
机构
[1] Chinese Acad Sci, Inst Atmospher Phys, State Key Lab Atmospher Boundary Layer Phys & Atm, Beijing 100029, Peoples R China
[2] Chinese Acad Sci, Inst Atmospher Phys, State Key Lab Numer Modeling Atmospher Sci & Geop, Beijing 100029, Peoples R China
[3] Chinese Acad Sci, Grad Univ, Beijing 100029, Peoples R China
基金
中国国家自然科学基金;
关键词
SPATIAL-DISTRIBUTION; UNITED-STATES; PART I; CLIMATE; PM2.5; SULFATE; VISIBILITY; INVENTORY; EMISSIONS; TRANSPORT;
D O I
10.1029/2012GL051428
中图分类号
P [天文学、地球科学];
学科分类号
07 ;
摘要
China has been experiencing increased concentrations of aerosols, commonly attributed to the large increases in emissions associated with the rapid economic development. We show by using a chemical transport model driven by the assimilated meteorological fields that the observed decadal-scale weakening of the East Asian summer monsoon also contributed to the increases in aerosols in China. We find that the simulated aerosol concentrations have strong negative correlations with the strength of the East Asian Summer monsoon. Accounting for sulfate, nitrate, ammonium, black carbon, and organic carbon aerosols, the summer surface-layer PM2.5 concentration averaged over eastern China (110 degrees-125 degrees E, 20 degrees-45 degrees N) can be 17.7% higher in the weakest monsoon years than in the strongest monsoon years. The weakening of the East Asian Summer monsoon increases aerosol concentrations mainly by the changes in atmospheric circulation (the convergence of air pollutants) in eastern China. Citation: Zhu, J., H. Liao, and J. Li (2012), Increases in aerosol concentrations over eastern China due to the decadal-scale weakening of the East Asian summer monsoon, Geophys. Res. Lett., 39, L09809, doi: 10.1029/2012GL051428.
引用
收藏
页数:6
相关论文
共 36 条
[1]   Sulfate formation in sea-salt aerosols: Constraints from oxygen isotopes [J].
Alexander, B ;
Park, RJ ;
Jacob, DJ ;
Li, QB ;
Yantosca, RM ;
Savarino, J ;
Lee, CCW ;
Thiemens, MH .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2005, 110 (D10) :1-12
[2]   Nitrate aerosols today and in 2030: a global simulation including aerosols and tropospheric ozone [J].
Bauer, S. E. ;
Koch, D. ;
Unger, N. ;
Metzger, S. M. ;
Shindell, D. T. ;
Streets, D. G. .
ATMOSPHERIC CHEMISTRY AND PHYSICS, 2007, 7 (19) :5043-5059
[3]   Anthropogenic Aerosols and the Weakening of the South Asian Summer Monsoon [J].
Bollasina, Massimo A. ;
Ming, Yi ;
Ramaswamy, V. .
SCIENCE, 2011, 334 (6055) :502-505
[4]   Spatial and seasonal distributions of carbonaceous aerosols over China [J].
Cao, J. J. ;
Lee, S. C. ;
Chow, J. C. ;
Watson, J. G. ;
Ho, K. F. ;
Zhang, R. J. ;
Jin, Z. D. ;
Shen, Z. X. ;
Chen, G. C. ;
Kang, Y. M. ;
Zou, S. C. ;
Zhang, L. Z. ;
Qi, S. H. ;
Dai, M. H. ;
Cheng, Y. ;
Hu, K. .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2007, 112 (D22)
[5]  
Chang CP, 2000, J CLIMATE, V13, P4310, DOI 10.1175/1520-0442(2000)013<4310:IAIVOT>2.0.CO
[6]  
2
[7]   Sensitivity of PM2.5 to climate in the Eastern US:: a modeling case study [J].
Dawson, J. P. ;
Adams, P. J. ;
Pandis, S. N. .
ATMOSPHERIC CHEMISTRY AND PHYSICS, 2007, 7 (16) :4295-4309
[8]   Inter-decadal variation of the summer precipitation in East China and its association with decreasing Asian summer monsoon. Part I: Observed evidences [J].
Ding, Yihui ;
Wang, Zunya ;
Sun, Ying .
INTERNATIONAL JOURNAL OF CLIMATOLOGY, 2008, 28 (09) :1139-1161
[9]   Concentration and chemical characteristics of PM2.5 in Beijing, China:: 2001-2002 [J].
Duan, FK ;
He, KB ;
Ma, YL ;
Yang, FM ;
Yu, XC ;
Cadle, SH ;
Chan, T ;
Mulawa, PA .
SCIENCE OF THE TOTAL ENVIRONMENT, 2006, 355 (1-3) :264-275
[10]   The impact of transpacific transport of mineral dust in the United States [J].
Fairlie, T. Duncan ;
Jacob, Daniel J. ;
Park, Rokjin J. .
ATMOSPHERIC ENVIRONMENT, 2007, 41 (06) :1251-1266