CO2 bubble behaviors and two-phase flow characteristics in single-serpentine sinusoidal corrugated channels of direct methanol fuel cell

被引:23
作者
Su, Xiaoqing [1 ]
Yuan, Wei [1 ]
Lu, Biaowu [1 ]
Zheng, Tianxiang [1 ]
Ke, Yuzhi [1 ]
Zhuang, Ziyi [1 ]
Zhao, Yonghao [1 ]
Tang, Yong [1 ]
Zhang, Shiwei [1 ,2 ]
机构
[1] South China Univ Technol, Sch Mech & Automot Engn, Guangzhou 510640, Guangdong, Peoples R China
[2] City Univ Hong Kong, Dept Mech Engn, Kowloon, Hong Kong, Peoples R China
基金
中国国家自然科学基金;
关键词
Direct methanol fuel cell; Two-phase flow; CO2; bubbles; Sinusoidal corrugated channel; Disturbance structure; Phase field; INTERFACIAL DYNAMICS; REACTANT TRANSPORT; MICROSCALE FLOW; FIELD DESIGNS; PERFORMANCE; ANODE; WATER; DMFC; FLUIDS; VISUALIZATION;
D O I
10.1016/j.jpowsour.2019.227621
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
Management of the produced carbon dioxide (CO2) is important to improve the performance of a liquid-feed direct methanol fuel cell (DMFC). This work investigates the CO2 bubble behaviors and the two-phase flow characteristics, using a single sinusoidal corrugated channel as the anode flow field. The magnitude and gradient of the fluid velocity in this channel is higher than the traditional straight pattern, as proven by tracking CO2 bubbles. The use of high magnitude and gradient of velocity enhances CO2 emission and fuel delivery, as well as increases the pressure drop. The vortices in the disturbance structure of the corrugated channel help uniformly deliver the reactants and separate bubbles away from the channel wall. Using excessive values of amplitude A and angular frequency W in the corrugated channel causes serious bubble deformation and extra energy consumption. The effect of disturbance structure is negligible with small values of these two parameters. The cell with a corrugated channel shows a higher performance at different feed rates and concentrations of the methanol fuel. The optimal value of A and W are respectively 0.1and 5. The visualization tests demonstrate that the appearance of CO2 bubbles in the corrugated channel is consistent with the simulation results.
引用
收藏
页数:13
相关论文
共 35 条
  • [21] Design and optimization of a novel sinusoidal corrugated channel for microfluidic fuel cell with gas-liquid two-phase flow model
    Ouyang, Tiancheng
    Liu, Wenjun
    Liu, Benlong
    Hu, Xiaoyi
    Shi, Xiaomin
    RENEWABLE ENERGY, 2023, 208 : 737 - 750
  • [22] Study on two-phase countercurrent flow and transport phenomenon in PEM of a direct methanol fuel cell
    Jiang Wang
    Mingheng Shi
    Science in China Series E, 2006, 49 : 102 - 114
  • [23] Study on two-phase countercurrent flow and transport phenomenon in PEM of a direct methanol fuel cell
    Wang, J
    Shi, MH
    SCIENCE IN CHINA SERIES E-TECHNOLOGICAL SCIENCES, 2006, 49 (01): : 102 - 114
  • [24] Study on two-phase countercurrent flow and transport phenomenon in PEM of a direct methanol fuel cell
    WANG Jiang & SHI Mingheng Department of Power Engineering
    Science in China(Series E:Technological Sciences), 2006, (01) : 102 - 114
  • [25] A TWO-PHASE FLOW STUDY ON CARBON DIOXIDE BUBBLES EVOLUTION IN DIRECT-METHANOL FUEL CELLS WITH DEGASSING CHANNELS
    Osman, Sameer
    Ahmed, Mahmoud
    PROCEEDINGS OF ASME 2021 INTERNATIONAL MECHANICAL ENGINEERING CONGRESS AND EXPOSITION (IMECE2021), VOL 8B, 2021,
  • [26] Investigation of CO2 bubble behavior and performance in air-breathing direct methanol fuel cells with spiral-patterned anode flow field
    Vasu, Vemuloori
    Srinivasulu, G. Naga
    Rao, Kammela Nagamalleswara
    THERMAL SCIENCE AND ENGINEERING PROGRESS, 2025, 59
  • [27] A three-dimensional two-phase flow model for a liquid-fed direct methanol fuel cell
    Ge, Jiabin
    Liu, Hongtan
    JOURNAL OF POWER SOURCES, 2007, 163 (02) : 907 - 915
  • [28] On two-phase flow patterns and transition criteria in aqueous methanol and CO2 mixtures in adiabatic, rectangular microchannels
    Weinmueller, C.
    Hotz, N.
    Mueller, A.
    Poulikakos, D.
    INTERNATIONAL JOURNAL OF MULTIPHASE FLOW, 2009, 35 (08) : 760 - 772
  • [29] Novel method for investigation of two-phase flow in liquid feed direct methanol fuel cells using an aqueous H2O2 solution
    Bewer, T
    Beckmann, T
    Dohle, H
    Mergel, J
    Stolten, D
    JOURNAL OF POWER SOURCES, 2004, 125 (01) : 1 - 9
  • [30] Flow resistance characteristics of two-phase CO2 with a large pressure gradient: Theoretical and experimental research
    Liu, Changchun
    Wu, Pengzhi
    Song, Fangzhi
    Jiang, Hua
    Huang, Linyuan
    Deng, Tiandiao
    Luo, Zhenmin
    INTERNATIONAL JOURNAL OF GREENHOUSE GAS CONTROL, 2022, 114