Levels of PCDD/FS in ambient air and soil in the vicinity of a municipal solid waste incinerator in Hsinchu

被引:82
作者
Cheng, PS [1 ]
Hsu, MS [1 ]
Ma, E [1 ]
Chou, U [1 ]
Ling, YC [1 ]
机构
[1] Natl Tsing Hua Univ, Dept Chem, Hsinchu 30043, Taiwan
关键词
dioxin; PCDD/Fs; MSWI; air; soil; PCA; HCA;
D O I
10.1016/S0045-6535(03)00474-0
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Levels of polychlorinated dibenzo-p-dioxins and dibenzofurans (PCDD/Fs) were determined in twenty-one ambient air samples, eight soil samples and two stack gas samples, collected near or in a municipal solid waste incinerator (MSWI) in Hsinchu, Taiwan. A systematic decrease of PCDD/Fs in the ambient air from the northeastern area was observed. PCDD/Fs levels measured in the ambient air range from 0.058 to 0.127 pg-TEQ/m(3). Higher PCDD/Fs levels in the ambient air were found during winter. In addition, PCDD/Fs levels measured in the soil range from 0.524 to 5.02 pg-TEQ/g d.m. Principal component analysis (PCA) and hierarchical cluster analysis (HCA) did not provide sufficient evidence that the environmental PCDD/Fs contamination was caused by emissions from the Hsinchu MSWL An unknown PCDD/Fs source was proposed using congener profile analysis and supported by both PCA and HCA. (C) 2003 Elsevier Ltd. All rights reserved.
引用
收藏
页码:1389 / 1396
页数:8
相关论文
共 16 条
  • [1] PCDD/PCDF from emission sources and ambient air in northeast Spain
    Abad, E
    Caixach, J
    Rivera, J
    [J]. CHEMOSPHERE, 1997, 35 (03) : 453 - 463
  • [2] [Anonymous], TO9A US EPA
  • [3] MULTIVARIATE STATISTICAL-ANALYSES OF PCDD AND PCDF LEVELS IN FISH, SEDIMENT, AND SOIL SAMPLES COLLECTED NEAR RESOURCE RECOVERY FACILITIES
    BAUER, KM
    CRAMER, PH
    STANLEY, JS
    FREDETTE, C
    GIGLINTO, TL
    [J]. CHEMOSPHERE, 1992, 25 (7-10) : 1441 - 1447
  • [4] Coutinho M, 2000, ORGANOHALOGEN COMPD, V46, P447
  • [5] *EPA ROC, 2000, EST PCDD F LEV INF A, P4
  • [6] *EPA ROC, 1990, CONSTR PROGR MUN SOL
  • [7] Sources of PCDD/PCDF and impact on the environment
    Fiedler, H
    [J]. CHEMOSPHERE, 1996, 32 (01) : 55 - 64
  • [8] Baseline contamination assessment for a new resource recovery facility in Germany .2. Atmospheric concentrations of PCDD/F
    Hippelein, M
    Kaupp, H
    Dorr, G
    McLachlan, M
    Hutzinger, O
    [J]. CHEMOSPHERE, 1996, 32 (08) : 1605 - 1616
  • [9] Testing the USA EPA's ISCST-Version 3 model on dioxins: a comparison of predicted and observed air and soil concentrations
    Lorber, M
    Eschenroeder, A
    Robinson, R
    [J]. ATMOSPHERIC ENVIRONMENT, 2000, 34 (23) : 3995 - 4010
  • [10] Relationships between dioxins in soil, air, ash, and emissions from a municipal solid waste incinerator emitting large amounts of dioxins
    Lorber, M
    Pinsky, P
    Gehring, P
    Braverman, C
    Winters, D
    Sovocool, W
    [J]. CHEMOSPHERE, 1998, 37 (9-12) : 2173 - 2197