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Performance analysis of VPSA process for separating N2O from adipic acid tail gas
被引:9
作者:
Wu, Tongbo
[1
]
Niu, Zhaoyang
[1
]
Feng, Li
[1
]
Yu, Xiuxin
[1
]
Liu, Bing
[1
]
Zhang, Donghui
[1
]
机构:
[1] Tianjin Univ, Sch Chem Engn & Technol, Res Ctr Chem Engn, Tianjin 300072, Peoples R China
关键词:
VPSA;
N2O separation;
Performance analysis;
Adipic acid tail gas;
NITROUS-OXIDE N2O;
ADSORPTION PROCESS;
CO2;
CAPTURE;
OPTIMIZATION;
SIMULATION;
CATALYST;
SYNGAS;
CARBON;
D O I:
10.1016/j.seppur.2020.117750
中图分类号:
TQ [化学工业];
学科分类号:
0817 ;
摘要:
A four-bed and six-bed vacuum pressure swing adsorption (VPSA) process with silical gel were proposed to separate and purify N2O from adipic acid tail gas (N2O/N-2/O-2 = 0.3933/0.5657/0.041 mol%) in nylon plants and then the N2O could be rectified to produce ultra-high purity N2O. The four-bed VPSA process was developed to study the relationship between vacuum pressure and simulation performances, the resulting recovery of N2O exceeds 90% with a purity over 95%. Meanwhile, the six-bed process was designed to explore the effects of vacuum and feed flow rate. The results indicated that a 95.55% purity N2O stream is attained for a process N2O recovery of 97.45%, when the feed flow rate was 1434.8 NL/s and vacuum pressure was 0.247 bar and N2O energy was 4.95 KJ/mol N2O respectively.
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页数:10
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