Correlation between the extinction spectrum of a single metal nanoparticle and its electron microscopy image

被引：71

作者：

Billaud, P. ^{[1
]}

Marhaba, S. ^{[1
]}

Cottancin, E. ^{[1
]}

Arnaud, L. ^{[1
]}

Bachelier, G. ^{[1
]}

Bonnet, C. ^{[1
]}

Del Fatti, N. ^{[1
]}

Lerme, J. ^{[1
]}

Vallee, F. ^{[1
]}

Vialle, J. -L. ^{[1
]}

Broyer, M. ^{[1
]}

Pellarin, M. ^{[1
]}

机构：

[1] Univ Lyon 1, CNRS, LASIM, UMR 5579, F-69622 Villeurbanne, France

来源：

JOURNAL OF PHYSICAL CHEMISTRY C | 2008年 / 112卷 / 04期

关键词：

D O I：

10.1021/jp076955m

中图分类号：

O64 [物理化学（理论化学）、化学物理学];

学科分类号：

070304 ; 081704 ;

摘要：

The absolute extinction cross-section spectrum of a single nanoparticle measured using spatial modulation spectroscopy (SMS) is correlated with its transmission electron microscopy (TEM) image. The sizes of quasi-spherical particles obtained by the two methods are found to be in good quantitative agreement. The possibilities opened up by combination of these methods for precise correlation of the optical response of a nanoobject with its geometry are illustrated in the case of a pair of interacting nanoparticles (dimer).

引用

页码：978 / 982

页数：5

共 22 条

[1] Morphology and growth of metal clusters in the gas phase:: A transition from spherical to ramified structures [J].

Alayan, R ;

Arnaud, L ;

Broyer, M ;

Cottancin, E ;

Lermé, J ;

Vialle, JL ;

Pellarin, M .

PHYSICAL REVIEW B, 2006, 73 (12)

[2] Direct measurement of the single-metal-cluster optical absorption -: art. no. 127401 [J].

Arbouet, A ;

Christofilos, D ;

Del Fatti, N ;

Vallée, F ;

Huntzinger, JR ;

Arnaud, L ;

Billaud, P ;

Broyer, M .

PHYSICAL REVIEW LETTERS, 2004, 93 (12) :127401-1

[3] Strongly interacting plasmon nanoparticle pairs: From dipole-dipole interaction to conductively coupled regime [J].

Atay, T ;

Song, JH ;

Nurmikko, AV .

NANO LETTERS, 2004, 4 (09) :1627-1631

[4] Photothermal heterodyne imaging of individual nonfluorescent nanoclusters and nanocrystals [J].

Berciaud, S ;

Cognet, L ;

Blab, GA ;

Lounis, B .

PHYSICAL REVIEW LETTERS, 2004, 93 (25)

[5] Optical extinction spectroscopy of single silver nanoparticles [J].

Billaud, P. ;

Huntzinger, J.-R. ;

Cottancin, E. ;

Lerme, J. ;

Pellarin, M. ;

Arnaud, L. ;

Broyer, M. ;

Del Fatti, N. ;

Vallee, F. .

EUROPEAN PHYSICAL JOURNAL D, 2007, 43 (1-3) :271-274

[6] Photothermal imaging of nanometer-sized metal particles among scatterers [J].

Boyer, D ;

Tamarat, P ;

Maali, A ;

Lounis, B ;

Orrit, M .

SCIENCE, 2002, 297 (5584) :1160-1163

[7] Optical frequency mixing at coupled gold nanoparticles [J].

Danckwerts, Matthias ;

Novotny, Lukas .

PHYSICAL REVIEW LETTERS, 2007, 98 (02)

[8] Relation between the optical properties of composite Si3N4 thin films with embedded Cu clusters and the clusters morphology:: Irradiation effects [J].

Girardeau, T ;

Camelio, S ;

Traverse, A ;

Lignou, F ;

Allain, J ;

Naudon, A ;

Guérin, P .

JOURNAL OF APPLIED PHYSICS, 2001, 90 (04) :1788-1794

[9] Correlating second harmonic optical responses of single Ag nanoparticles with morphology [J].

Jin, RC ;

Jureller, JE ;

Kim, HY ;

Scherer, NF .

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2005, 127 (36) :12482-12483

[10] OPTICAL CONSTANTS OF NOBLE METALS [J].

JOHNSON, PB ;

CHRISTY, RW .

PHYSICAL REVIEW B, 1972, 6 (12) :4370-4379

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