Atomic structure and magnetic moments in cluster-assembled nanocomposite Fe/Cu films

被引:21
作者
Baker, S. H. [1 ]
Asaduzzaman, A. M. [1 ]
Roy, M. [1 ]
Gurman, S. J. [1 ]
Binns, C. [1 ]
Blackman, J. A. [1 ,2 ]
Xie, Y. [2 ]
机构
[1] Univ Leicester, Dept Phys & Astron, Leicester LE1 7RH, Leics, England
[2] Univ Reading, Dept Phys, Reading RG6 6AF, Berks, England
来源
PHYSICAL REVIEW B | 2008年 / 78卷 / 01期
关键词
D O I
10.1103/PhysRevB.78.014422
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
The atomic structure and net magnetic moments in nanosized Fe clusters embedded in Cu were determined as a function of cluster filling fraction by extended x-ray-absorption fine structure (EXAFS) and magnetometry measurements, respectively. Below the percolation threshold (similar to 25%), the Fe clusters have an fcc structure with a lattice parameter of 3.58 +/- 0.02 angstrom and are ferromagnetic with a net atomic magnetic moment of 0.4-0.9 mu(B). Spin polarized electronic structure calculations were also performed on Fe core/Cu shell systems to investigate the magnetic behavior as a function of lattice spacing; the calculated moments correlate well with experiment.
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页数:10
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共 60 条
  • [1] NEUTRON DIFFRACTION DETERMINATION OF ANTIFERROMAGNETISM IN FACE-CENTERED CUBIC (GAMMA) IRON
    ABRAHAMS, SC
    GUTTMAN, L
    KASPER, JS
    [J]. PHYSICAL REVIEW, 1962, 127 (06): : 2052 - &
  • [2] ANDERSEN OK, 1977, PHYSICA B & C, V86, P249, DOI 10.1016/0378-4363(77)90303-5
  • [3] EXPLICIT, 1ST-PRINCIPLES TIGHT-BINDING THEORY
    ANDERSEN, OK
    JEPSEN, O
    [J]. PHYSICAL REVIEW LETTERS, 1984, 53 (27) : 2571 - 2574
  • [4] ILLUSTRATION OF THE LINEAR-MUFFIN-TIN-ORBITAL TIGHT-BINDING REPRESENTATION - COMPACT ORBITALS AND CHARGE-DENSITY IN SI
    ANDERSEN, OK
    PAWLOWSKA, Z
    JEPSEN, O
    [J]. PHYSICAL REVIEW B, 1986, 34 (08): : 5253 - 5269
  • [5] Tight-binding molecular-dynamics study of ferromagnetic clusters
    Andriotis, AN
    Menon, M
    [J]. PHYSICAL REVIEW B, 1998, 57 (16) : 10069 - 10081
  • [6] LATTICE-PARAMETER DEPENDENCE OF FERROMAGNETISM IN BCC AND FCC IRON
    BAGAYOKO, D
    CALLAWAY, J
    [J]. PHYSICAL REVIEW B, 1983, 28 (10) : 5419 - 5422
  • [7] The construction of a gas aggregation source for the preparation of size-selected nanoscale transition metal clusters
    Baker, SH
    Thornton, SC
    Edmonds, KW
    Maher, MJ
    Norris, C
    Binns, C
    [J]. REVIEW OF SCIENTIFIC INSTRUMENTS, 2000, 71 (08) : 3178 - 3183
  • [8] Atomic structure in magnetic cluster assembled Fe/Co films as determined from extended absorption fine structure
    Baker, SH
    Roy, M
    Louch, S
    Binns, C
    [J]. JOURNAL OF PHYSICS-CONDENSED MATTER, 2006, 18 (08) : 2385 - 2399
  • [9] Enhancements in magnetic moments of exposed and Co-coated Fe nanoclusters as a function of cluster size
    Baker, SH
    Binns, C
    Edmonds, KW
    Maher, MJ
    Thornton, SC
    Louch, S
    Dhesi, SS
    [J]. JOURNAL OF MAGNETISM AND MAGNETIC MATERIALS, 2002, 247 (01) : 19 - 25
  • [10] MAGNETIC-MOMENTS OF IRON CLUSTERS WITH 25 TO 700 ATOMS AND THEIR DEPENDENCE ON TEMPERATURE
    BILLAS, IML
    BECKER, JA
    CHATELAIN, A
    DEHEER, WA
    [J]. PHYSICAL REVIEW LETTERS, 1993, 71 (24) : 4067 - 4070