C60 adsorption onto the one-atomic-layer In films on Si(111) surface

被引:11
作者
Gruznev, D. V. [1 ]
Matetskiy, A. V. [1 ]
Gvozd, I. V. [1 ]
Zotov, A. V. [1 ,2 ,3 ]
Saranin, A. A. [1 ,2 ]
机构
[1] Inst Automat & Control Proc, Vladivostok 690041, Russia
[2] Far Eastern State Univ, Fac Phys & Engn, Vladivostok 690000, Russia
[3] Vladivostok State Univ Econ & Serv, Dept Elect, Vladivostok 690600, Russia
基金
俄罗斯基础研究基金会;
关键词
Atom-solid interactions; Silicon; Indium; Fullerene; Surface structure; Morphology; Roughness; Topography; Scanning tunneling microscopy (STM); ROOT 3-IN SURFACE; STM; TEMPERATURE; SUBSTRATE; GROWTH;
D O I
10.1016/j.susc.2011.07.008
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
We have studied C-60 adsorption onto the In-induced Si(111) reconstructions, Si(111)2x2-In. Si(111)-hex-root 7 x root 3-In, and Si(111)-rec-root 7 x root 3-In, which all represent essentially one-atomic-layer In films residing atop a bulk-like Si(111) substrate. The reconstructions have various In densities, incorporating 0.75, 1.0, and 1.2 ML of In, respectively. We have found that C-60 adsorption onto these reconstruction is accompanied by the mass transport within In atomic layer, which is manifested by developing the domains of a more dense In/Si(111) reconstruction on the surface in between C-60. This observation provides a direct evidence for the displacement of In atoms from beneath C-60 to the surrounding surface area. The plausible driven force of the C-60-induced In displacement is a tendency of C-60 to change relatively modest bonding with In layer to a more stronger bond with Si(111) substrate. (C) 2011 Elsevier B.V. All rights reserved.
引用
收藏
页码:1951 / 1955
页数:5
相关论文
共 37 条
[1]   Adsorption and motion of C60 molecules on the Pb-covered Si(111) surface [J].
Chang, Shih-Hsin ;
Hwang, Ing-Shouh ;
Fang, Chung-Kai ;
Tsong, Tien T. .
PHYSICAL REVIEW B, 2008, 77 (15)
[2]   Core-level photoemission study of additional In adsorption on the Si(111)√3x√3-In surface -: art. no. 035414 [J].
Cho, SW ;
Nakamura, K ;
Koh, H ;
Choi, WH ;
Whang, CN ;
Yeom, HW .
PHYSICAL REVIEW B, 2003, 67 (03)
[3]   X-ray-diffraction characterization of Pt(111) surface nanopatterning induced by C60 adsorption [J].
Felici, R ;
Pedio, M ;
Borgatti, F ;
Iannotta, S ;
Capozi, M ;
Ciullo, G ;
Stierle, A .
NATURE MATERIALS, 2005, 4 (09) :688-692
[4]   Scanning tunneling microscopy studies of C60 monolayers on Au(111) [J].
Gardener, J. A. ;
Briggs, G. A. D. ;
Castell, M. R. .
PHYSICAL REVIEW B, 2009, 80 (23)
[5]   INTRAMOLECULAR STRUCTURES OF C60 MOLECULES ADSORBED ON THE CU(111)-(1X1) SURFACE [J].
HASHIZUME, T ;
MOTAI, K ;
WANG, XD ;
SHINOHARA, H ;
SAITO, Y ;
MARUYAMA, Y ;
OHNO, K ;
KAWAZOE, Y ;
NISHINA, Y ;
PICKERING, HW ;
KUK, Y ;
SAKURAI, T .
PHYSICAL REVIEW LETTERS, 1993, 71 (18) :2959-2962
[6]   Looking underneath fullerenes on Au(110): Formation of dimples in the substrate [J].
Hinterstein, M. ;
Torrelles, X. ;
Felici, R. ;
Rius, J. ;
Huang, M. ;
Fabris, S. ;
Fuess, H. ;
Pedio, M. .
PHYSICAL REVIEW B, 2008, 77 (15)
[7]   Aperiodic incommensurate phase of a C60 monolayer on Ag(100) -: art. no. 245414 [J].
Hsu, CL ;
Pai, WW .
PHYSICAL REVIEW B, 2003, 68 (24)
[8]   Surface reconstructions of In on Si(111) [J].
Kraft, J ;
Ramsey, MG ;
Netzer, FP .
PHYSICAL REVIEW B, 1997, 55 (08) :5384-5393
[9]   C-60 - BUCKMINSTERFULLERENE [J].
KROTO, HW ;
HEATH, JR ;
OBRIEN, SC ;
CURL, RF ;
SMALLEY, RE .
NATURE, 1985, 318 (6042) :162-163
[10]   Origin of Moireacute structures in C60 on Pb(111) and their effect on molecular energy levels [J].
Li, H. I. ;
Franke, K. J. ;
Pascual, J. I. ;
Bruch, L. W. ;
Diehl, R. D. .
PHYSICAL REVIEW B, 2009, 80 (08)