Hybrid Bilayer WSe2-CH3NH3PbI3 Organolead Halide Perovskite as a High-Performance Photodetector

被引：96

作者：

Lu, Junpeng ^{[1
,2
,3
]}

Carvalho, Alexandra ^{[2
,3
]}

Liu, Hongwei ^{[4
]}

Lim, Sharon Xiaodai ^{[1
]}

Castro Neto, Antonio H. ^{[1
,2
,3
]}

Sow, Chorng Haur ^{[1
,2
,3
]}

机构：

[1] Natl Univ Singapore, Dept Phys, 2 Sci Dr 3, Singapore 117542, Singapore

[2] Natl Univ Singapore, Ctr Adv Mat 2D, 6 Sci Dr 2, Singapore 117546, Singapore

[3] Natl Univ Singapore, Graphene Res Ctr, 6 Sci Dr 2, Singapore 117546, Singapore

[4] ASTAR, Inst Mat Res & Engn, 2 Fusionopolis Way Innovis,08-03, Singapore 138634, Singapore

来源：

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION | 2016年 / 55卷 / 39期

关键词：

2D transition-metal-dichalcogenides; laser healing; optoelectronic devices; perovskite; SOLAR-CELLS; MOS2; CH3NH3PBI3; DIODES;

D O I：

10.1002/anie.201603557

中图分类号：

O6 [化学];

学科分类号：

0703 ;

摘要：

A high-performance 2D photodetector based on a bilayer structure comprising a WSe2 monolayer and CH3NH3PbI3 organolead halide perovskite is reported. High performance is realized by modification of the WSe2 monolayer with laser healing and perovskite functionalization. After modification, the output of the device was three orders of magnitude better than the pristine device; the performance is superior to that of most of the 2D photodetectors based on transition-metal-dichalcogenides (TMDs). This result indicates that combinatory TMDs-halide perovskite hybrids can be promising building blocks in optoelectronics.

引用

页码：11945 / 11949

页数：5

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