Propane-fuelled microtubular solid oxide fuel cell stack electrically connected by an anodic rectangular window

被引:8
作者
Liang, Bo [1 ,2 ]
Yao, Yue [1 ]
Guo, Jin [1 ]
Yang, Huazheng [1 ]
Liang, Jiajiang [1 ]
Zhao, Zhijiang [2 ]
Wu, Gang [2 ]
Zhan, Yuedong [2 ]
Zhao, Xiaobo [1 ]
Tao, Tao [1 ]
Yao, Yingbang [1 ]
Lu, Shengguo [1 ]
Zhao, Ruirui [3 ]
机构
[1] Guangdong Univ Technol, Sch Mat & Energy, Guangdong Prov Key Lab Funct Soft Condensed Matte, Guangzhou 510006, Peoples R China
[2] ISOFC Dynam Co Ltd, Foshan, Peoples R China
[3] South China Normal Univ, Sch Chem, Guangzhou 510006, Peoples R China
基金
国家重点研发计划; 中国国家自然科学基金;
关键词
Microtubular solid oxide fuel cell; Catalytic partial oxidation; Carbon deposition; Crack; MICRO-TUBULAR SOFC; ELECTROCHEMICAL PERFORMANCE; HYDROGEN-PRODUCTION; OXIDATION;
D O I
10.1016/j.apenergy.2021.118404
中图分类号
TE [石油、天然气工业]; TK [能源与动力工程];
学科分类号
0807 ; 0820 ;
摘要
A current collecting window (0.4 cm(2)), without an electrolyte and cathode, is located in the middle of an anode and connected electrically to the cathode of another microtubular solid oxide fuel cell (MTSOFC) when building a short stack. No apparent open-circuit voltage (OCV) drops were observed during 31 thermal cycles for an 8-cell stack using H-2 and syngas. Furthermore, 24.1, 53.6 and 103.5 W power levels are achieved employing this current collecting mode at 700 C for an 8, 10 and 20-cell stack, respectively. The propane-fuelled 8-cell stack has a maximum power density (MPD) of 0.30 W cm(-2) when integrated with a catalytic partial oxidation (CPOX) reformer, at a flow rate of 0.32 g min(-1) of propane. A Pt-Ru nanoparticle is fabricated by impregnation treatment of the alumina honeycomb ceramic support. The Pt-based catalyst, with an average size of similar to 10.0 nm, is well distributed on the surface of the honeycomb ceramic channel. Moreover, Pt-Ru/Al2O3, as a CPOX catalyst, ex-hibits high propane conversions (94.2%) at 700 C.
引用
收藏
页数:8
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