An integrated nanocatalyst combining enzymatic and metal-organic framework catalysts for cascade degradation of organophosphate nerve agents

被引:41
作者
Li, Haibin [1 ]
Ma, Li [1 ]
Zhou, Liya [1 ]
Gao, Jing [1 ]
Huang, Zhihong [1 ]
He, Ying [1 ]
Jiang, Yanjun [1 ,2 ]
机构
[1] Hebei Univ Technol, Sch Chem Engn & Technol, 8 Guangrong Rd, Tianjin 300130, Peoples R China
[2] Hebei Univ Technol, Natl Local Joint Engn Lab Energy Conservat Chem P, Tianjin 300130, Peoples R China
关键词
FACILE SYNTHESIS; NITROPHENOL REDUCTION; NANOPARTICLES; MIL-100(FE); IMMOBILIZATION; PERFORMANCE; SIMULANTS; LIPASE;
D O I
10.1039/c8cc06727a
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
An integrated nanocatalyst (INC), denoted OPH@MIL-100(Fe), was synthesized by immobilizing a biocatalyst onto a metal-organic framework (MOF)-based catalyst, which can cascadingly degrade organophosphate nerve agents to 4-aminophenol (4-AP) and result in a sharp decrease of their toxicity up to 208-fold.
引用
收藏
页码:10754 / 10757
页数:4
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