Enhanced Efficiency of MAPbI3 Perovskite Solar Cells with FAPbX3 Perovskite Quantum Dots

被引:30
作者
Chen, Lung-Chien [1 ]
Tien, Ching-Ho [1 ]
Tseng, Zong-Liang [2 ,3 ]
Ruan, Jun-Hao [1 ]
机构
[1] Natl Taipei Univ Technol, Dept Electroopt Engn, Taipei 10608, Taiwan
[2] Ming Chi Univ Technol, Dept Elect Engn, New Taipei 24301, Taiwan
[3] Ming Chi Univ Technol, Organ Elect Res Ctr, New Taipei 24301, Taiwan
关键词
solar cells; perovskite; quantum dots; MAPbI(3); FAPbX(3); EXCITON BINDING-ENERGY; HALIDE PEROVSKITES; HIGHLY EFFICIENT; METHYLAMMONIUM; BR;
D O I
10.3390/nano9010121
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
We describe a method to enhance power conversion efficiency (PCE) of MAPbI(3) perovskite solar cell by inserting a FAPbX(3) perovskite quantum dots (QD-FAPbX(3)) layer. The MAPbI(3) and QD-FAPbX(3) layers were prepared using a simple, rapid spin-coating method in a nitrogen-filled glove box. The solar cell structure consists of ITO/PEDOT:PSS/MAPbI(3)/QD-FAPbX(3)/C-60/Ag, where PEDOT:PSS, MAPbI(3), QD-FAPbX(3), and C-60 were used as the hole transport layer, light-absorbing layer, absorption enhance layer, and electron transport layer, respectively. The MAPbI(3)/QD-FAPbX(3) solar cells exhibit a PCE of 7.59%, an open circuit voltage (Voc) of 0.9 V, a short-circuit current density (Jsc) of 17.4 mA/cm(2), and a fill factor (FF) of 48.6%, respectively.
引用
收藏
页数:8
相关论文
共 20 条
  • [1] [Anonymous], Best Research Cell Efficiencies
  • [2] Preparation and Characteristics of MAPbBr3 Perovskite Quantum Dots on NiOx Film and Application for High Transparent Solar Cells
    Chen, Lung-Chien
    Lee, Kuan-Lin
    Huang, Chun-Yuan
    Lin, Jia-Ching
    Tseng, Zong-Liang
    [J]. MICROMACHINES, 2018, 9 (05)
  • [3] Effect of Different CH3NH3PbI3 Morphologies on Photovoltaic Properties o Perovskite Solar Cells
    Chen, Lung-Chien
    Lee, Kuan-Lin
    Wu, Wen-Ti
    Hsu, Chien-Feng
    Tseng, Zong-Liang
    Sun, Xiao Hong
    Kao, Yu-Ting
    [J]. NANOSCALE RESEARCH LETTERS, 2018, 13
  • [4] An ultrasonic synthesis method for high-luminance perovskite quantum dots
    Chen, Lung-Chien
    Tseng, Zong-Liang
    Chen, Shih-You
    Yang, Shengyi
    [J]. CERAMICS INTERNATIONAL, 2017, 43 (17) : 16032 - 16035
  • [5] Organometallic Halide Perovskites: Sharp Optical Absorption Edge and Its Relation to Photovoltaic Performance
    De Wolf, Stefaan
    Holovsky, Jakub
    Moon, Soo-Jin
    Loeper, Philipp
    Niesen, Bjoern
    Ledinsky, Martin
    Haug, Franz-Josef
    Yum, Jun-Ho
    Ballif, Christophe
    [J]. JOURNAL OF PHYSICAL CHEMISTRY LETTERS, 2014, 5 (06): : 1035 - 1039
  • [6] Determination of the exciton binding energy and effective masses for methylammonium and formamidinium lead tri-halide perovskite semiconductors
    Galkowski, Krzysztof
    Mitioglu, Anatolie
    Miyata, Atsuhiko
    Plochocka, Paulina
    Portugall, Oliver
    Eperon, Giles E.
    Wang, Jacob Tse-Wei
    Stergiopoulos, Thomas
    Stranks, Samuel D.
    Snaith, Henry J.
    Nicholas, Robin J.
    [J]. ENERGY & ENVIRONMENTAL SCIENCE, 2016, 9 (03) : 962 - 970
  • [7] Dependence of halide composition on the stability of highly efficient all-inorganic cesium lead halide perovskite quantum dot solar cells
    Ghosh, Dibyendu
    Ali, Md. Yusuf
    Chaudhary, Dhirendra K.
    Bhattacharyya, Sayan
    [J]. SOLAR ENERGY MATERIALS AND SOLAR CELLS, 2018, 185 : 28 - 35
  • [8] Hybrid PbS Quantum-Dot-in-Perovskite for High-Efficiency Perovskite Solar Cell
    Han, Jianhua
    Luo, Songping
    Yin, Xuewen
    Zhou, Yu
    Nan, Hui
    Li, Jianbao
    Li, Xin
    Oron, Dan
    Shen, Heping
    Lin, Hong
    [J]. SMALL, 2018, 14 (31)
  • [9] 6.5% efficient perovskite quantum-dot-sensitized solar cell
    Im, Jeong-Hyeok
    Lee, Chang-Ryul
    Lee, Jin-Wook
    Park, Sang-Won
    Park, Nam-Gyu
    [J]. NANOSCALE, 2011, 3 (10) : 4088 - 4093
  • [10] Organometal Halide Perovskites as Visible-Light Sensitizers for Photovoltaic Cells
    Kojima, Akihiro
    Teshima, Kenjiro
    Shirai, Yasuo
    Miyasaka, Tsutomu
    [J]. JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2009, 131 (17) : 6050 - +