Synergies between BECCS and Biochar-Maximizing Carbon Sequestration Potential by Recycling Wood Ash

被引:46
作者
Buss, Wolfram [1 ]
Jansson, Stina [2 ]
Wurzer, Christian [1 ]
Masek, Ondrej [1 ]
机构
[1] Univ Edinburgh, UK Biochar Res Ctr, Sch GeoSci, Crew Bldg,Alexander Crum Brown Rd, Edinburgh EH9 3FF, Midlothian, Scotland
[2] Umea Univ, Dept Chem, Linnaeus Vag 6, SE-90187 Umea, Sweden
关键词
CO2; abatement; Carbon stability; Fixed carbon; Thermogravimetric analysis; Combustion; Negative emission technology; STABILITY; SLUDGE;
D O I
10.1021/acssuschemeng.8b05871
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Bioenergy carbon capture and storage (BECCS) and biochar are key carbon-negative technologies. In this study, synergies between these technologies were explored by using ash from wood combustion, a byproduct from BECCS, as an additive (0, 5, 10, 20, and 50 wt %) in biochar production (wood pyrolysis at 450 degrees C). The addition of wood ash catalyzed biochar formation and increased the yield of fixed carbon (FC) (per dry, ash-free feedstock), i.e., the sequestrable carbon per spruce wood input. At the highest ash addition (50%), 45% less wood was needed to yield the same amount of FC. Since the land area available for growing biomass is becoming scarcer, our approach significantly increases biochar's potential to sequester carbon. However, increasing the feedstock ash content results in less feedstock carbon available for conversion into FC. Consequently, the yield of FC per pyrolysis run (based on dry feedstock) in the 50% ash-amended material was lower than in the control. An economic analysis showed that the 20% ash-amended biochar brings the biggest cost savings over the control with a 15% decrease in CO2-abatement costs. Biochar-ash composites increase the carbon sequestration potential of biochar significantly, reduce the CO2-abatement costs, and recycle nutrients which can result in increased plant growth in turn and more biomass for BECCS, bringing synergies for BECCS and biochar deployment.
引用
收藏
页码:4204 / 4209
页数:11
相关论文
共 35 条
  • [1] Modified method for proximate analysis of biochars
    Aller, Deborah
    Bakshi, Santanu
    Laird, David A.
    [J]. JOURNAL OF ANALYTICAL AND APPLIED PYROLYSIS, 2017, 124 : 335 - 342
  • [2] Interactions between biochar stability and soil organisms: review and research needs
    Ameloot, N.
    Graber, E. R.
    Verheijen, F. G. A.
    De Neve, S.
    [J]. EUROPEAN JOURNAL OF SOIL SCIENCE, 2013, 64 (04) : 379 - 390
  • [3] [Anonymous], 2013, CLIM CHANG 2013 PHYS
  • [4] [Anonymous], 2015, BIOCHAR ENV MANAGEME
  • [5] The art, science, and technology of charcoal production
    Antal, MJ
    Gronli, M
    [J]. INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH, 2003, 42 (08) : 1619 - 1640
  • [6] ASTM, 1990, D176284 ASTM INT, P292
  • [7] Budai A., 2013, INT BIOCHAR INITIATI
  • [8] Unexplored potential of novel biochar-ash composites for use as organo-mineral fertilizers
    Buss, Wolfram
    Jansson, Stina
    Masek, Ondrej
    [J]. JOURNAL OF CLEANER PRODUCTION, 2019, 208 : 960 - 967
  • [9] Mobile organic compounds in biochar - A potential source of contamination - Phytotoxic effects on cress seed (Lepidium sativum) germination
    Buss, Wolfram
    Masek, Ondrej
    [J]. JOURNAL OF ENVIRONMENTAL MANAGEMENT, 2014, 137 : 111 - 119
  • [10] Pyrolysis biochar systems, balance between bioenergy and carbon sequestration
    Crombie, Kyle
    Masek, Ondrej
    [J]. GLOBAL CHANGE BIOLOGY BIOENERGY, 2015, 7 (02): : 349 - 361