Unidirectional spin density wave state in metallic (Sr1-xLax)2IrO4

被引:38
作者
Chen, Xiang [1 ,2 ]
Schmehr, Julian L. [2 ]
Islam, Zahirul [3 ]
Porter, Zach [4 ]
Zoghlin, Eli [2 ]
Finkelstein, Kenneth [5 ]
Ruff, Jacob P. C. [5 ]
Wilson, Stephen D. [2 ]
机构
[1] Boston Coll, Dept Phys, Chestnut Hill, MA 02467 USA
[2] Univ Calif Santa Barbara, Dept Mat, Santa Barbara, CA 93106 USA
[3] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA
[4] Univ Calif Santa Barbara, Dept Phys, Santa Barbara, CA 93106 USA
[5] Cornell Univ, Cornell High Energy Synchrotron Source, Ithaca, NY 14853 USA
基金
美国国家科学基金会; 美国国家卫生研究院;
关键词
MAGNETIC CORRELATIONS; PHASE;
D O I
10.1038/s41467-017-02647-1
中图分类号
O [数理科学和化学]; P [天文学、地球科学]; Q [生物科学]; N [自然科学总论];
学科分类号
07 ; 0710 ; 09 ;
摘要
Materials that exhibit both strong spin-orbit coupling and electron correlation effects are predicted to host numerous new electronic states. One prominent example is the J(eff) = 1/2 Mott state in Sr2IrO4, where introducing carriers is predicted to manifest high temperature superconductivity analogous to the S = 1/2 Mott state of La2CuO4. While bulk super-conductivity currently remains elusive, anomalous quasiparticle behaviors paralleling those in the cuprates such as pseudogap formation and the formation of a d-wave gap are observed upon electron-doping Sr2IrO4. Here we establish a magnetic parallel between electron-doped Sr2IrO4 and hole-doped La2CuO4 by unveiling a spin density wave state in electron-doped Sr2IrO4. Our magnetic resonant X-ray scattering data reveal the presence of an incommensurate magnetic state reminiscent of the diagonal spin density wave state observed in the monolayer cuprate (La1-xSrx)(2)CuO4. This link supports the conjecture that the quenched Mott phases in electron-doped Sr2IrO4 and hole-doped La2CuO4 support common competing electronic phases.
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页数:7
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共 38 条
[1]  
Battisti I, 2017, NAT PHYS, V13, P21, DOI [10.1038/nphys3894, 10.1038/NPHYS3894]
[2]   Magnetic neutron scattering in hole-doped cuprate superconductors [J].
Birgeneau, Robert J. ;
Stock, Chris ;
Tranquada, John M. ;
Yamada, Kazuyoshi .
JOURNAL OF THE PHYSICAL SOCIETY OF JAPAN, 2006, 75 (11)
[3]   Locking of iridium magnetic moments to the correlated rotation of oxygen octahedra in Sr2IrO4 revealed by x-ray resonant scattering [J].
Boseggia, S. ;
Walker, H. C. ;
Vale, J. ;
Springell, R. ;
Feng, Z. ;
Perry, R. S. ;
Sala, M. Moretti ;
Ronnow, H. M. ;
Collins, S. P. ;
McMorrow, D. F. .
JOURNAL OF PHYSICS-CONDENSED MATTER, 2013, 25 (42)
[4]   Weak ferromagnetism, metal-to-nonmetal transition, and negative differential resistivity in single-crystal Sr2IrO4 [J].
Cao, G ;
Bolivar, J ;
McCall, S ;
Crow, JE ;
Guertin, RP .
PHYSICAL REVIEW B, 1998, 57 (18) :R11039-R11042
[5]   Hallmarks of the Mott-metal crossover in the hole-doped pseudospin-1/2 Mott insulator Sr2IrO4 [J].
Cao, Yue ;
Wang, Qiang ;
Waugh, Justin A. ;
Reber, Theodore J. ;
Li, Haoxiang ;
Zhou, Xiaoqing ;
Parham, Stephen ;
Park, S-R ;
Plumb, Nicholas C. ;
Rotenberg, Eli ;
Bostwick, Aaron ;
Denlinger, Jonathan D. ;
Qi, Tongfei ;
Hermele, Michael A. ;
Cao, Gang ;
Dessau, Daniel S. .
NATURE COMMUNICATIONS, 2016, 7
[6]   Influence of electron doping on the ground state of (Sr1-xLax)2IrO4 [J].
Chen, Xiang ;
Hogan, Tom ;
Walkup, D. ;
Zhou, Wenwen ;
Pokharel, M. ;
Yao, Mengliang ;
Tian, Wei ;
Ward, Thomas Z. ;
Zhao, Y. ;
Parshall, D. ;
Opeil, C. ;
Lynn, J. W. ;
Madhavan, Vidya ;
Wilson, Stephen D. .
PHYSICAL REVIEW B, 2015, 92 (07)
[7]   Spin-orbit coupling in iridium-based 5d compounds probed by x-ray absorption spectroscopy [J].
Clancy, J. P. ;
Chen, N. ;
Kim, C. Y. ;
Chen, W. F. ;
Plumb, K. W. ;
Jeon, B. C. ;
Noh, T. W. ;
Kim, Young-June .
PHYSICAL REVIEW B, 2012, 86 (19)
[8]   STRUCTURAL AND MAGNETIC STUDIES OF SR2IRO4 [J].
CRAWFORD, MK ;
SUBRAMANIAN, MA ;
HARLOW, RL ;
FERNANDEZBACA, JA ;
WANG, ZR ;
JOHNSTON, DC .
PHYSICAL REVIEW B, 1994, 49 (13) :9198-9201
[9]   Collapse of the Mott Gap and Emergence of a Nodal Liquid in Lightly Doped Sr2IrO4 [J].
de la Torre, A. ;
Walker, S. McKeown ;
Bruno, F. Y. ;
Ricco, S. ;
Wang, Z. ;
Lezama, I. Gutierrez ;
Scheerer, G. ;
Giriat, G. ;
Jaccard, D. ;
Berthod, C. ;
Kim, T. K. ;
Hoesch, M. ;
Hunter, E. C. ;
Perry, R. S. ;
Tamai, A. ;
Baumberger, F. .
PHYSICAL REVIEW LETTERS, 2015, 115 (17)
[10]  
Dean MPM, 2016, NAT MATER, V15, P601, DOI [10.1038/NMAT4641, 10.1038/nmat4641]