Modeling Amine Aerosol Growth in the Absorber and Water Wash

被引：12

作者：

Kang, Jia-Lin ^{[1
]}

Zhang, Yue ^{[2
]}

Fulk, Steven ^{[2
]}

Rochelle, Gary T. ^{[2
]}

机构：

[1] Natl Tsing Hua Univ, Dept Chem Engn, Hsinchu, Taiwan

[2] Univ Texas Austin, McKetta Dept Chem Engn, Texas Carbon Management Program, 200 E Dean Keeton St,C0400, Austin, TX 78712 USA

来源：

13TH INTERNATIONAL CONFERENCE ON GREENHOUSE GAS CONTROL TECHNOLOGIES, GHGT-13 | 2017年 / 114卷

关键词：

Amine; CO2; capture; Aerosol; modeling;

D O I：

10.1016/j.egypro.2017.03.1241

中图分类号：

X [环境科学、安全科学];

学科分类号：

08 ; 0830 ;

摘要：

This study has developed a multi-layer model to estimate concentration gradients inside aerosol and aerosol growth. The results show that piperazine (PZ) aerosol grows from 0.1 um to 3.2 mu m in the absorber and up to 9.6 mu m in the water wash with 10(7) particles/cm(3). Aerosol can be assumed to be well-mixed in the absorber and water wash. The PZ gradient in the aerosol is negligible because of the small aerosol diameter. Larger particle number concentration results in smaller drops. Aerosol growth is controlled by PZ mass transfer in the absorber and by water mass transfer in the water wash. More volatile amine should provide faster growth in the absorber. (C) 2017 The Authors. Published by Elsevier Ltd.

引用

页码：959 / 976

页数：18

共 6 条

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