Photolytic reactors: Similitude in Taylor-Couette and channel flows

被引:7
作者
Forney, LJ [1 ]
Pierson, JA
机构
[1] Georgia Tech, Sch Chem Engn, Atlanta, GA 30332 USA
[2] Georgia Tech Res Inst, Atlanta, GA 30332 USA
关键词
D O I
10.1002/aic.690490519
中图分类号
TQ [化学工业];
学科分类号
0817 ;
摘要
A similarity law is proposed for the yield from laminar photolytic reactors. In particular, the yield from a fast photolytic reaction is considered in the following three distinctly different reactor geometries: a square channel, an annular gap between concentric cylinders, and Taylor - Couette flow. The similarity law, based on the assumption of a self similar product concentration profile, demonstrates that the reaction rate can best be described with either zero (small A) or first-order (large A) kinetics. Here, the distinction between both cases is determined by the radiation penetration depth, A. Other geometric parameters affecting scale-up are also discussed.
引用
收藏
页码:1285 / 1292
页数:8
相关论文
共 26 条
[1]   Prediction of mass transfer rates in spatially periodic flows [J].
Baier, G ;
Grateful, TM ;
Graham, MD ;
Lightfoot, EN .
CHEMICAL ENGINEERING SCIENCE, 1999, 54 (03) :343-355
[2]  
Bird R B., 2002, Transportphenomena
[3]  
BLATCHLEY ER, 1995, J ENVIRON ENG-ASCE, V121, P258
[4]   Process modeling of ultraviolet disinfection [J].
Blatchley, ER ;
Do-Quang, Z ;
Janex, ML ;
Laîné, JM .
WATER SCIENCE AND TECHNOLOGY, 1998, 38 (06) :63-69
[5]   Integrated UV disinfection model based on particle tracking [J].
Chiu, K ;
Lyn, DA ;
Savoye, P ;
Blatchley, ER .
JOURNAL OF ENVIRONMENTAL ENGINEERING-ASCE, 1999, 125 (01) :7-16
[6]  
CONGDINE DM, 1976, VANNOSTRANDS SCI ENC, P1764
[7]   EFFECTS OF ULTRAVIOLET IRRADIATION ON LARGE POPULATIONS OF CERTAIN WATER-BORNE BACTERIA IN MOTION .1. THE DEVELOPMENT OF ADEQUATE AGITATION TO PROVIDE AN EFFECTIVE EXPOSURE PERIOD [J].
CORTELYOU, JR ;
MCWHINNIE, MA ;
RIDDIFORD, MS ;
SEMRAD, JE .
APPLIED MICROBIOLOGY, 1954, 2 (04) :227-235
[8]   PRIMARY PROCESSES IN PHOTOLYSIS OF IODIDE ION IN AQUEOUS SOLUTION [J].
DAINTON, FS ;
LOGAN, SR .
PROCEEDINGS OF THE ROYAL SOCIETY OF LONDON SERIES A-MATHEMATICAL AND PHYSICAL SCIENCES, 1965, 287 (1410) :281-&
[9]   Optimum photolysis in Taylor-Couette flow [J].
Forney, LJ ;
Pierson, JA .
AICHE JOURNAL, 2003, 49 (03) :727-733
[10]  
Incropera FrankP., 2002, INTRO HEAT TRANSFER, V4th