Enhanced electrical conductivity in graphene-copper multilayer composite

被引:19
作者
Pan, Chaochao [1 ]
Gaur, Anand P. S. [1 ]
Lynn, Matthew [2 ]
Olson, Madison P. [1 ]
Ouyang, Gaoyuan [3 ]
Cui, Jun [1 ,3 ]
机构
[1] Iowa State Univ, Dept Mat Sci & Engn, Ames, IA 50011 USA
[2] Ames Lab, Sensit Instrument Facil, Ames, IA 50011 USA
[3] Ames Lab, Div Mat Sci & Engn, Ames, IA 50011 USA
关键词
ELECTRONIC-STRUCTURE; MECHANICAL-PROPERTIES; CARBON NANOTUBES; HIGH-QUALITY; MICROSTRUCTURE; RESISTIVITY; STRENGTH; FILMS;
D O I
10.1063/5.0073879
中图分类号
TB3 [工程材料学];
学科分类号
0805 ; 080502 ;
摘要
For many years, researchers have been trying to make a material more conductive than silver by incorporating carbon nanotubes or graphene into copper to form a composite material. However, after a decade-long effort, only a few groups reported successful results, raising concerns about the feasibility of this composite approach. Here, we report our effort to validate the multilayer graphene-copper composite approach for improving electrical conductivity. We demonstrate that, with an estimated 0.008 vol. % graphene addition, copper's electrical conductivity was improved to 104.2% of International Annealed Copper Standard (IACS) at room temperature. If the copper substrate used to make the multilayer composite is discounted using the parallel resistance model, the conductivity is calculated to be 185% IACS. This result could be further improved if the thickness of the copper layers can be further reduced. (c) 2022 Author(s). All article content, except where otherwise noted, is licensed under a Creative Commons Attribution (CC BY) license (http://creativecommons.org/licenses/by/4.0/).
引用
收藏
页数:6
相关论文
共 49 条
  • [1] Sorting carbon nanotubes by electronic structure using density differentiation
    Arnold, Michael S.
    Green, Alexander A.
    Hulvat, James F.
    Stupp, Samuel I.
    Hersam, Mark C.
    [J]. NATURE NANOTECHNOLOGY, 2006, 1 (01) : 60 - 65
  • [2] Graphene: synthesis and applications
    Avouris, Phaedon
    Dimitrakopoulos, Christos
    [J]. MATERIALS TODAY, 2012, 15 (03) : 86 - 97
  • [3] Electrical properties and applications of carbon nanotube structures
    Bandaru, Prabhakar R.
    [J]. JOURNAL OF NANOSCIENCE AND NANOTECHNOLOGY, 2007, 7 (4-5) : 1239 - 1267
  • [4] Experimental studies of the electronic structure of graphene
    Bostwick, Aaron
    McChesney, Jessica
    Ohta, Taisuke
    Rotenberg, Eli
    Seyller, Thomas
    Horn, Karsten
    [J]. PROGRESS IN SURFACE SCIENCE, 2009, 84 (11-12) : 380 - 413
  • [5] Single-step deposition of high-mobility graphene at reduced temperatures
    Boyd, D. A.
    Lin, W. -H.
    Hsu, C. -C.
    Teague, M. L.
    Chen, C. -C.
    Lo, Y. -Y.
    Chan, W. -Y.
    Su, W. -B.
    Cheng, T. -C.
    Chang, C. -S.
    Wu, C. -I.
    Yeh, N. -C.
    [J]. NATURE COMMUNICATIONS, 2015, 6
  • [6] Ultrahigh Electrical Conductivity of Graphene Embedded in Metals
    Cao, Mu
    Xiong, Ding-Bang
    Yang, Li
    Li, Shuaishuai
    Xie, Yiqun
    Guo, Qiang
    Li, Zhiqiong
    Adams, Horst
    Gu, Jiajun
    Fan, Tongxiang
    Zhang, Xiaohui
    Zhang, Di
    [J]. ADVANCED FUNCTIONAL MATERIALS, 2019, 29 (17)
  • [7] Aligning graphene in bulk copper: Nacre-inspired nanolaminated architecture coupled with in-situ processing for enhanced mechanical properties and high electrical conductivity
    Cao, Mu
    Xiong, Ding-Bang
    Tan, Zhanqiu
    Ji, Gang
    Amin-Ahmadi, Behnam
    Guo, Qiang
    Fan, Genlian
    Guo, Cuiping
    Li, Zhiqiang
    Zhang, Di
    [J]. CARBON, 2017, 117 : 65 - 74
  • [8] First-principles study of metal adatom adsorption on graphene
    Chan, Kevin T.
    Neaton, J. B.
    Cohen, Marvin L.
    [J]. PHYSICAL REVIEW B, 2008, 77 (23):
  • [9] Effects of graphene content on the microstructure and properties of copper matrix composites
    Chen, Fanyan
    Ying, Jiamin
    Wang, Yifei
    Du, Shiyu
    Liu, Zhaoping
    Huang, Qing
    [J]. CARBON, 2016, 96 : 836 - 842
  • [10] Fabrication of in-situ grown graphene reinforced Cu matrix composites
    Chen, Yakun
    Zhang, Xiang
    Liu, Enzuo
    He, Chunnian
    Shi, Chunsheng
    Li, Jiajun
    Nash, Philip
    Zhao, Naiqin
    [J]. SCIENTIFIC REPORTS, 2016, 6