The dielectric function of PbS quantum dots in a glass matrix

被引:44
作者
Moreels, Iwan [1 ]
Kruschke, Detlef [2 ]
Glas, Peter [3 ]
Tomm, Jens W. [4 ]
机构
[1] Ist Italiano Tecnol, I-16163 Genoa, Italy
[2] Inst Angew Photon eV, D-12489 Berlin, Germany
[3] Inst Sci Instruments GmbH, D-12489 Berlin, Germany
[4] Max Born Inst Nichtlineare Opt & Kurzpulsspektros, D-12489 Berlin, Germany
关键词
Sulfur compounds - Nanocrystals - Iterative methods - IV-VI semiconductors - Lead compounds - Semiconductor quantum dots;
D O I
10.1364/OME.2.000496
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
The dielectric function of PbS quantum dots (Qdots) with diameters of 3.5-5.0 nm in glass matrix is determined from transmission measurements by Maxwell-Garnett effective medium theory combined with iterative Kramers-Kronig analysis. The algorithm used provides real and imaginary part of the dielectric function in the 200-1800 nm spectral range, for both Qdot-doped glasses as well as the PbS Qdots alone. The latter data are compared with the results obtained from colloidal PbS quantum dots and, within the limits of the experimental error, agreement is found. (C) 2012 Optical Society of America
引用
收藏
页码:496 / 500
页数:5
相关论文
共 13 条
[1]   QUANTUM CONFINEMENT OF PBS MICROCRYSTALS IN GLASS [J].
BORRELLI, NF ;
SMITH, DW .
JOURNAL OF NON-CRYSTALLINE SOLIDS, 1994, 180 (01) :25-31
[2]  
FOX KE, 1982, PHYS CHEM GLASSES, V23, P169
[3]   PbS quantum-dot doped grasses as saturable absorbers for mode locking of a Cr:forsterite laser [J].
Guerreiro, PT ;
Ten, S ;
Borrelli, NF ;
Butty, J ;
Jabbour, GE ;
Peyghambarian, N .
APPLIED PHYSICS LETTERS, 1997, 71 (12) :1595-1597
[4]   Hybrid solar cells using PbS nanoparticles [J].
Gunes, Serap ;
Fritz, Karolina P. ;
Neugebauer, Helmut ;
Sariciftci, Niyazi Serdar ;
Kumar, Sandeep ;
Scholes, Gregory D. .
SOLAR ENERGY MATERIALS AND SOLAR CELLS, 2007, 91 (05) :420-423
[5]   Infrared quantum dots for liquid-phase thermometry in silicon [J].
Kim, M. ;
Yoda, M. .
MEASUREMENT SCIENCE AND TECHNOLOGY, 2011, 22 (08)
[6]   Efficient infrared electroluminescent devices using solution-processed colloidal quantum dots [J].
Konstantatos, G ;
Huang, CJ ;
Levina, L ;
Lu, ZH ;
Sargent, EH .
ADVANCED FUNCTIONAL MATERIALS, 2005, 15 (11) :1865-1869
[7]   Efficient infrared-emitting PbS quantum dots grown on DNA and stable in aqueous solution and blood plasma [J].
Levina, L ;
Sukhovatkin, W ;
Musikhin, S ;
Cauchi, S ;
Nisman, R ;
Bazett-Jones, DP ;
Sargent, EH .
ADVANCED MATERIALS, 2005, 17 (15) :1854-+
[8]   Solution-processed PbS quantum dot infrared photodetectors and photovoltaics [J].
McDonald, SA ;
Konstantatos, G ;
Zhang, SG ;
Cyr, PW ;
Klem, EJD ;
Levina, L ;
Sargent, EH .
NATURE MATERIALS, 2005, 4 (02) :138-142
[9]   Dielectric function of colloidal lead chalcogenide quantum dots obtained by a Kramers-Kronig analysis of the absorbance spectrum [J].
Moreels, Iwan ;
Allan, Guy ;
De Geyter, Bram ;
Wirtz, Ludger ;
Delerue, Christophe ;
Hens, Zeger .
PHYSICAL REVIEW B, 2010, 81 (23)
[10]   Size-Dependent Optical Properties of Colloidal PbS Quantum Dots [J].
Moreels, Iwan ;
Lambert, Karel ;
Smeets, Dries ;
De Muynck, David ;
Nollet, Tom ;
Martins, Jose C. ;
Vanhaecke, Frank ;
Vantomme, Andre ;
Delerue, Christophe ;
Allan, Guy ;
Hens, Zeger .
ACS NANO, 2009, 3 (10) :3023-3030