[1] Soot and smoke aerosol contain black carbon, which absorbs solar radiation. These aerosols may reduce the overall negative climate forcing of anthropogenic aerosols by absorbing radiation that might otherwise be scattered back to space. They may also reduce overall cloudiness, an effect termed the "semidirect'' effect, which is thought to enhance climate warming. Here, we evaluate the climate forcing associated with black carbon and other aerosols using the concept of "relaxed forcing,'' which is the forcing associated with two simulations using fixed sea surface temperatures. The consideration of longwave perturbations associated with the relaxed forcing leads to a diminished or even negative semidirect effect associated with absorbing aerosols rather than an enhanced warming. The overall forcing depends significantly on the altitude of injection of the aerosols because higher-altitude injections tend to enhance the negative longwave forcing. In addition, high-altitude injection of absorbing aerosols can increase cloudiness at lower altitudes where temperatures, in general, may decrease.
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Arizona State Univ, Sch Earth & Space Explorat, Tempe, AZ 85287 USA
Arizona State Univ, Dept Chem & Biochem, Tempe, AZ 85287 USAArizona State Univ, Sch Earth & Space Explorat, Tempe, AZ 85287 USA
Adachi, Kouji
Chung, Serena H.
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Washington State Univ, Dept Civil & Environm Engn, Pullman, WA 99164 USAArizona State Univ, Sch Earth & Space Explorat, Tempe, AZ 85287 USA
Chung, Serena H.
Buseck, Peter R.
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Arizona State Univ, Sch Earth & Space Explorat, Tempe, AZ 85287 USA
Arizona State Univ, Dept Chem & Biochem, Tempe, AZ 85287 USAArizona State Univ, Sch Earth & Space Explorat, Tempe, AZ 85287 USA
机构:
Condensed Matter Laboratory, Department of Physics, Kansas State University, Manhattan, KS 66506-2601, United StatesCondensed Matter Laboratory, Department of Physics, Kansas State University, Manhattan, KS 66506-2601, United States
Sorensen, C.M.
Hageman, W.B.
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Condensed Matter Laboratory, Department of Physics, Kansas State University, Manhattan, KS 66506-2601, United StatesCondensed Matter Laboratory, Department of Physics, Kansas State University, Manhattan, KS 66506-2601, United States
Hageman, W.B.
Rush, T.J.
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Condensed Matter Laboratory, Department of Physics, Kansas State University, Manhattan, KS 66506-2601, United StatesCondensed Matter Laboratory, Department of Physics, Kansas State University, Manhattan, KS 66506-2601, United States
Rush, T.J.
Huang, H.
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Condensed Matter Laboratory, Department of Physics, Kansas State University, Manhattan, KS 66506-2601, United StatesCondensed Matter Laboratory, Department of Physics, Kansas State University, Manhattan, KS 66506-2601, United States
Huang, H.
Oh, C.
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Condensed Matter Laboratory, Department of Physics, Kansas State University, Manhattan, KS 66506-2601, United StatesCondensed Matter Laboratory, Department of Physics, Kansas State University, Manhattan, KS 66506-2601, United States