Life cycle assessment of hydrogen production from a high temperature electrolysis process coupled to a high temperature gas nuclear reactor

被引:50
作者
Giraldi, Mario R. [1 ]
Francois, Juan-Luis [1 ]
Martin-del-Campo, Cecilia [1 ]
机构
[1] Univ Nacl Autonoma Mexico, Fac Ingn, Dept Sistemas Energet, Jiutepec 62550, Morelos, Mexico
关键词
Hydrogen production; LCA; GHG; Nuclear energy chain; High temperature electrolysis; High temperature gas reactor; ENVIRONMENTAL-IMPACT;
D O I
10.1016/j.ijhydene.2015.01.093
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
The life cycle analysis (LCA) is a versatile tool to evaluate process and production systems, and is useful to compare environmental burdens. For the purposes of this LCA, a high temperature electrolysis process was coupled to a high temperature gas nuclear reactor. The system function is the production of hydrogen using electricity and heat from nuclear power, with a functional unit of 1 kg of hydrogen, at the plant gate. The product system consists of the following steps: (i) the extraction and manufacturing of raw materials (upstream flows), (ii) the electrolytic cell fabrication, (iii) the nuclear fuel cycle, and, (iv) the hydrogen production plant. Particular attention was paid to those processes where there was limited information available on inventory data, for example mining and processing of rare earth metals, and electrolytic cell assembly, which are the primary components of a hydrogen generation plant. The environmental impact assessment focuses on the emissions of greenhouse gases (GHGs), as related to global warming. Additionally, other environmental loads, to complete the environmental profile of the product system, were included. The results were low GHGs emissions, with a value of 416 g of CO(2)eq kg(-1)H(2). As to the process components, the electrolytic cell showed the highest environmental impact. Copyright (C) 2015, Hydrogen Energy Publications, LLC. Published by Elsevier Ltd. All rights reserved.
引用
收藏
页码:4019 / 4033
页数:15
相关论文
共 45 条
[1]  
[Anonymous], 2006, ISO 14040 2006 ENV M
[2]  
[Anonymous], 1996, P TECHN COMM M JOH S
[3]  
Bailey L, 2009, THESIS U TORONTO
[4]   Life cycle assessment of fuel cell-based APUs [J].
Baratto, F ;
Diwekar, UM .
JOURNAL OF POWER SOURCES, 2005, 139 (1-2) :188-196
[5]   Value Choices in Life Cycle Impact Assessment of Stressors Causing Human Health Damage [J].
De Schryver, An M. ;
van Zelm, Rosalie ;
Humbert, Sebastien ;
Pfister, Stephan ;
McKone, Thomas E. ;
Huijbregts, Mark A. J. .
JOURNAL OF INDUSTRIAL ECOLOGY, 2011, 15 (05) :796-815
[6]   Comparative life cycle assessment of three biohydrogen pathways [J].
Djomo, Sylvestre Njakou ;
Blumberga, Dagnija .
BIORESOURCE TECHNOLOGY, 2011, 102 (03) :2684-2694
[7]  
Eccleston KL, 2007, THESIS U ST ANDREWS
[8]   Human health damages due to ionising radiation in life cycle impact assessment [J].
Frischknecht, R ;
Braunschweig, A ;
Hofstetter, P ;
Suter, P .
ENVIRONMENTAL IMPACT ASSESSMENT REVIEW, 2000, 20 (02) :159-189
[9]   Metrics of climate change: Assessing radiative forcing and emission indices [J].
Fuglestvedt, JS ;
Berntsen, TK ;
Godal, O ;
Sausen, R ;
Shine, KP ;
Skodvin, T .
CLIMATIC CHANGE, 2003, 58 (03) :267-331
[10]   Life cycle greenhouse gases emission analysis of hydrogen production from S-I thermochemical process coupled to a high temperature nuclear reactor [J].
Giraldi, Mario R. ;
Francois, Juan-Luis ;
Castro-Uriegas, Daniel .
INTERNATIONAL JOURNAL OF HYDROGEN ENERGY, 2012, 37 (19) :13933-13942