Fabrication of high-performance MXene-based all-solid-state flexible microsupercapacitor based on a facile scratch method

被引:51
作者
Li, Peng [1 ]
Shi, Wenhui [2 ]
Liu, Wenxian [1 ]
Chen, Yafei [1 ]
Xu, Xilian [1 ]
Ye, Shaofeng [1 ]
Yin, Ruilian [1 ]
Zhang, Lin [1 ]
Xu, Lixin [1 ]
Cao, Xiehong [1 ,3 ,4 ]
机构
[1] Zhejiang Univ Technol, Coll Mat Sci & Engn, Hangzhou 310014, Zhejiang, Peoples R China
[2] Zhejiang Univ Technol, Ocean Coll, Ctr Membrane Separat & Water Sci & Technol, Hangzhou 310014, Zhejiang, Peoples R China
[3] Zhejiang Univ Technol, State Key Lab Breeding Base Green Chem Synth Tech, Hangzhou 310014, Zhejiang, Peoples R China
[4] Xian Univ Technol, Inst Adv Electrochem Energy, Xian 710048, Shaanxi, Peoples R China
基金
中国国家自然科学基金;
关键词
microsupercapacitors; MXenes; two-dimensional materials; all-solid-state flexible supercapacitors; interdigital electrode patterns; REDUCED GRAPHENE OXIDE; MICRO-SUPERCAPACITORS; CARBON; COMPOSITES; ELECTRODES; PAPER; INTERCALATION; CAPACITANCE; NANOARRAYS; NANOSHEETS;
D O I
10.1088/1361-6528/aadad4
中图分类号
TB3 [工程材料学];
学科分类号
0805 ; 080502 ;
摘要
MXenes have emerged as promising electrode materials for microsupercapacitors (MSCs) owing to their high volumetric and areal capacitances. In addition to the development of novel electrode materials, fabrication of interdigital electrodes is another key to realize high-performance MSCs. Herein, we demonstrate the patterning of few-layered Ti3C2Tx nanosheets on various substrates for MSCs by a facile, fast, and nearly zero-cost 'scratch' strategy. The fabricated Ti3C2Tx-based all-solid-state MSC achieves a high areal capacitance of 25.5 mF cm(-2), which benefits from the unique layered structure and high electrical conductivity of the electrode. The fabricated planar MSC also delivers good cycling stability and excellent flexibility. Moreover, our fabrication strategy can be readily extended to other composite films for MSCs and become potential micropower sources for miniaturized electronic devices.
引用
收藏
页数:10
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