Designed Redox Ions Pairs imprinted photocatalyst of Fe3+@PoPD/TiO2/HNTs for enhanced photocatalytic activity

被引：8

作者：

Tian, Xiaohua ^{[1
]}

Dai, Jiangdong ^{[2
]}

Zhu, Zhi ^{[2
]}

Yan, Yongsheng ^{[2
]}

Huo, Pengwei ^{[2
]}

机构：

[1] Jiangsu Univ, Sch Mat Sci & Engn, Zhenjiang, Jiangsu, Peoples R China

[2] Jiangsu Univ, Inst Green Chem & Chem Technol, Sch Chem & Chem Engn, Zhenjiang 212013, Jiangsu, Peoples R China

来源：

MATERIALS TECHNOLOGY | 2020年 / 35卷 / 13-14期

基金：

中国国家自然科学基金; 中国博士后科学基金;

关键词：

Redox Ions Pairs; Imprinted photocatalyst; Fe3+@PoPD; TiO2; HNTs; Tetracycline degradation; FERRITE COMPOSITE NANOPARTICLES; GRAPHITIC CARBON NITRIDE; FLY-ASH CENOSPHERES; VISIBLE-LIGHT; ANTIMICROBIAL ACTIVITY; MAGNETIC CORE; DOPED TIO2; PERFORMANCE; PHOTODEGRADATION; DEGRADATION;

D O I：

10.1080/10667857.2019.1704471

中图分类号：

T [工业技术];

学科分类号：

08 ;

摘要：

In this study, Fe3+@PoPD/TiO2/HNTs composite photocatalyst was successfully prepared by sol-gel method and ion-imprinting technique. The composite photocatalysts were characterised by X-ray diffraction (XRD), scanning electron microscopy (SEM), transmission electron microscopy (TEM), ultraviolet X-ray photoelectron spectroscopy (XPS) and ultraviolet-visible diffuse reflectance spectroscopy (UV-vis DRS). The photocatalytic activity of the composite photocatalyst was studied by simulating the degradation of tetracycline under sunlight. The results showed that the prepared composite photocatalyst had obvious activity for tetracycline degradation under simulated solar irradiation, and Fe3+@PoPD/TiO2/HNTs-1 had the best performance. The photodegradation rate can reach 91% in 90 min. This work may provide a promising approach for wastewater treatment by utilisation of ion imprinting technique and increasing photocatalytic performance of TiO2.

引用

页码：843 / 852

页数：10

共 46 条

[1] NGQD active sites as effective collectors of charge carriers for improving the photocatalytic performance of Z-scheme g-C3N4/Bi2WO6 heterojunctions [J].

Che, Huinan ;

Liu, Chunbo ;

Hu, Wei ;

Hu, Hao ;

Li, Jinqiao ;

Dou, Jianying ;

Shi, Weidong ;

Li, Chunmei ;

Dong, Hongjun .

CATALYSIS SCIENCE & TECHNOLOGY, 2018, 8 (02) :622-631

[2] Bimodal mesoporous TiO2-P25 composite thick films with high photocatalytic activity and improved structural integrity [J].

Chen, Yongjun ;

Dionysiou, Dionysios D. .

APPLIED CATALYSIS B-ENVIRONMENTAL, 2008, 80 (1-2) :147-155

[3] Adsorption and photodegradation of methylene blue on TiO2-halloysite adsorbents [J].

Du, Yuanyuan ;

Zheng, Pengwu .

KOREAN JOURNAL OF CHEMICAL ENGINEERING, 2014, 31 (11) :2051-2056

[4] Preparation molecular/ions imprinted photocatalysts of La3+@POPD/TiO2/fly-ash cenospheres: Preferential photodegradation of TCs antibiotics [J].

Huo, Pengwei ;

Lu, Ziyang ;

Liu, Xinlin ;

Xiaolin, Liu ;

Gao, Xun ;

Pan, Jianming ;

Wu, Di ;

Ying, Jun ;

Li, Huaming ;

Yan, Yongsheng .

CHEMICAL ENGINEERING JOURNAL, 2012, 198 :73-80

[5] Enhanced photodegradation of antibiotics solution under visible light with Fe2+/Fe3+ immobilized on TiO2/fly-ash cenospheres by using ions imprinting technology [J].

Huo, Pengwei ;

Lu, Ziyang ;

Wang, Huiqin ;

Pan, Jianming ;

Li, Huaming ;

Wu, Xiangyang ;

Huang, Weihong ;

Yan, Yongsheng .

CHEMICAL ENGINEERING JOURNAL, 2011, 172 (2-3) :615-622

[6] A new visible light active multifunctional ternary composite based on TiO2-In2O3 nanocrystals heterojunction decorated porous graphitic carbon nitride for photocatalytic treatment of hazardous pollutant and H2 evolution [J].

Jiang, Zhifeng ;

Jiang, Deli ;

Yan, Zaoxue ;

Liu, Dong ;

Qian, Kun ;

Xie, Jimin .

APPLIED CATALYSIS B-ENVIRONMENTAL, 2015, 170 :195-205

[7] Endowing single-electron-trapped oxygen vacancy self-modified titanium dioxide with visible-light photocatalytic activity by grafting Fe(III) nanocluster [J].

Li, Haiyan ;

Ren, Fengzhu ;

Liu, Jinfeng ;

Wang, Qinglong ;

Li, Qiuye ;

Yang, Jianjun ;

Wang, Yuanxu .

APPLIED CATALYSIS B-ENVIRONMENTAL, 2015, 172 :37-45

[8] Monolithically integrated stretchable photonics [J].

Li, Lan ;

Lin, Hongtao ;

Qiao, Shutao ;

Huang, Yi-Zhong ;

Li, Jun-Ying ;

Michon, Jerome ;

Gu, Tian ;

Alosno-Ramos, Carlos ;

Vivien, Laurent ;

Yadav, Anupama ;

Richardson, Kathleen ;

Lu, Nanshu ;

Hu, Juejun .

LIGHT-SCIENCE & APPLICATIONS, 2018, 7 :17138-17138

[9] Microwave-assisted synthesis of selective degradation photocatalyst by surface molecular imprinting method for the degradation of tetracycline onto Cl-TiO2 [J].

Liu, Xinlin ;

Lv, Peng ;

Yao, Guanxin ;

Ma, Changchang ;

Huo, Pengwei ;

Yan, Yongsheng .

CHEMICAL ENGINEERING JOURNAL, 2013, 217 :398-406

[10] In situ synthesis of C-TiO2/g-C3N4 heterojunction nanocomposite as highly visible light active photocatalyst originated from effective interfacial charge transfer [J].

Lu, Zhao ;

Zeng, Lei ;

Song, Wulin ;

Qin, Ziyu ;

Zeng, Dawen ;

Xie, Changsheng .

APPLIED CATALYSIS B-ENVIRONMENTAL, 2017, 202 :489-499

← 1 2 3 4 5 →