Reduced biomass burning emissions reconcile conflicting estimates of the post-2006 atmospheric methane budget

被引:134
作者
Worden, John R. [1 ]
Bloom, A. Anthony [1 ]
Pandey, Sudhanshu [2 ,3 ]
Jiang, Zhe [1 ,4 ]
Worden, Helen M. [4 ]
Walker, Thomas W. [1 ]
Houweling, Sander [2 ,3 ,5 ]
Rockmann, Thomas [2 ]
机构
[1] CALTECH, Jet Prop Lab, 4800 Oak Grove Dr, Pasadena, CA 91109 USA
[2] Univ Utrecht, Inst Marine & Atmospher Res Utrecht, Utrecht, Netherlands
[3] SRON Netherlands Inst Space Res, Utrecht, Netherlands
[4] Natl Ctr Atmospher Res, Boulder, CO 80301 USA
[5] Vrije Univ Amsterdam, Dept Earth Sci, Amsterdam, Netherlands
来源
NATURE COMMUNICATIONS | 2017年 / 8卷
基金
美国国家航空航天局; 加拿大自然科学与工程研究理事会; 美国国家科学基金会;
关键词
GLOBAL FIRE EMISSIONS; NATURAL-GAS PRODUCTION; FOSSIL-FUEL; DECADAL TRENDS; CLIMATE-CHANGE; CH4; EMISSIONS; CO EMISSIONS; BURNED AREA; AIR-QUALITY; MOPITT;
D O I
10.1038/s41467-017-02246-0
中图分类号
O [数理科学和化学]; P [天文学、地球科学]; Q [生物科学]; N [自然科学总论];
学科分类号
07 ; 0710 ; 09 ;
摘要
Several viable but conflicting explanations have been proposed to explain the recent similar to 8 p.p.b. per year increase in atmospheric methane after 2006, equivalent to net emissions increase of similar to 25 Tg CH4 per year. A concurrent increase in atmospheric ethane implicates a fossil source; a concurrent decrease in the heavy isotope content of methane points toward a biogenic source, while other studies propose a decrease in the chemical sink (OH). Here we show that biomass burning emissions of methane decreased by 3.7 (+/- 1.4) Tg CH4 per year from the 2001-2007 to the 2008-2014 time periods using satellite measurements of CO and CH4, nearly twice the decrease expected from prior estimates. After updating both the total and isotopic budgets for atmospheric methane with these revised biomass burning emissions (and assuming no change to the chemical sink), we find that fossil fuels contribute between 12-19 Tg CH4 per year to the recent atmospheric methane increase, thus reconciling the isotopic-and ethane-based results.
引用
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页数:11
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