Optimal conditions for NV- center formation in type-1b diamond studied using photoluminescence and positron annihilation spectroscopies

被引:48
作者
Botsoa, J. [1 ,2 ]
Sauvage, T. [1 ]
Adam, M-P. [2 ]
Desgardin, P. [1 ]
Leoni, E. [1 ]
Courtois, B. [1 ]
Treussart, F. [2 ]
Barthe, M-F. [1 ]
机构
[1] CNRS, UPR 3079, F-45071 Orleans, France
[2] Ecole Normale Super, CNRS, UMR 8537, Lab Photon Quant & Mol, F-94235 Cachan, France
来源
PHYSICAL REVIEW B | 2011年 / 84卷 / 12期
关键词
TRAPPING RATES; DIVACANCIES; VACANCIES; SPINS; BEAM;
D O I
10.1103/PhysRevB.84.125209
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
We studied the parameters to optimize the production of negatively charged nitrogen-vacancy color centers (NV-) in type-1b single crystal diamond using proton irradiation followed by thermal annealing under vacuum. Several samples were treated under different irradiation and annealing conditions and characterized by slow positron beam Doppler-broadening and photoluminescence (PL) spectroscopies. At high proton fluences another complex vacancy defect appears limiting the formation of NV-. Concentrations as high as 2.3 x 10(18) cm(-3) of NV- have been estimated from PL measurements. Furthermore, we inferred the trapping coefficient of positrons by NV-. This study brings insight into the production of a high concentration of NV- in diamond, which is of utmost importance in ultrasensitive magnetometry and quantum hybrid systems applications.
引用
收藏
页数:6
相关论文
共 24 条
[1]   Broadband magnetometry by infrared-absorption detection of nitrogen-vacancy ensembles in diamond [J].
Acosta, V. M. ;
Bauch, E. ;
Jarmola, A. ;
Zipp, L. J. ;
Ledbetter, M. P. ;
Budker, D. .
APPLIED PHYSICS LETTERS, 2010, 97 (17)
[2]   The diamond age of spintronics - Quantum electronic devices that harness the spins of electrons might one day enable room-temperature quantum computers - made of diamond [J].
Awschalom, David D. ;
Epstein, Ryan ;
Hanson, Ronald .
SCIENTIFIC AMERICAN, 2007, 297 (04) :84-+
[3]   Nanoscale imaging magnetometry with diamond spins under ambient conditions [J].
Balasubramanian, Gopalakrishnan ;
Chan, I. Y. ;
Kolesov, Roman ;
Al-Hmoud, Mohannad ;
Tisler, Julia ;
Shin, Chang ;
Kim, Changdong ;
Wojcik, Aleksander ;
Hemmer, Philip R. ;
Krueger, Anke ;
Hanke, Tobias ;
Leitenstorfer, Alfred ;
Bratschitsch, Rudolf ;
Jelezko, Fedor ;
Wrachtrup, Joerg .
NATURE, 2008, 455 (7213) :648-U46
[4]  
Chang HC, 2010, NANODIAMONDS: APPLICATIONS IN BIOLOGY AND NANOSCALE MEDICINE, P127, DOI 10.1007/978-1-4419-0531-4_6
[5]   Mass production and dynamic imaging of fluorescent nanodiamonds [J].
Chang, Yi-Ren ;
Lee, Hsu-Yang ;
Chen, Kowa ;
Chang, Chun-Chieh ;
Tsai, Dung-Sheng ;
Fu, Chi-Cheng ;
Lim, Tsong-Shin ;
Tzeng, Yan-Kai ;
Fang, Chia-Yi ;
Han, Chau-Chung ;
Chang, Huan-Cheng ;
Fann, Wunshain .
NATURE NANOTECHNOLOGY, 2008, 3 (05) :284-288
[6]   VACANCY-RELATED CENTERS IN DIAMOND [J].
DAVIES, G ;
LAWSON, SC ;
COLLINS, AT ;
MAINWOOD, A ;
SHARP, SJ .
PHYSICAL REVIEW B, 1992, 46 (20) :13157-13170
[7]   Slow positron beam facility in Orleans [J].
Desgardin, P ;
Liszkay, L ;
Barthe, MF ;
Henry, L ;
Briaud, J ;
Saillard, M ;
Lepolotec, L ;
Corbel, C ;
Blondiaux, G ;
Colder, A ;
Marie, P ;
Levalois, M .
POSITRON ANNIHILATION - ICPA-12, 2001, 363-3 :523-525
[8]   Photoluminescent nanodiamonds: Comparison of the photoluminescence saturation properties of the NV color center and a cyanine dye at the single emitter level, and study of the color center concentration under different preparation conditions [J].
Faklaris, Orestis ;
Botsoa, Jacques ;
Sauvage, Thierry ;
Roch, Jean-Francois ;
Treussart, Francois .
DIAMOND AND RELATED MATERIALS, 2010, 19 (7-9) :988-995
[9]   A slow positron beam study of natural and synthetic diamonds [J].
Fischer, CG ;
Connell, SH ;
Coleman, PG ;
Malik, F ;
Britton, DT ;
Sellschop, JPF .
APPLIED SURFACE SCIENCE, 1999, 149 (1-4) :221-226
[10]   Cavity QED Based on Collective Magnetic Dipole Coupling: Spin Ensembles as Hybrid Two-Level Systems [J].
Imamoglu, Atac .
PHYSICAL REVIEW LETTERS, 2009, 102 (08)