Ultrafast pump-probe force microscopy with nanoscale resolution

被引：77

作者：

Jahng, Junghoon ^{[1
]}

Brocious, Jordan ^{[1
]}

Fishman, Dmitry A. ^{[2
]}

Yampolsky, Steven ^{[2
]}

Nowak, Derek ^{[3
]}

Huang, Fei ^{[4
]}

Apkarian, Vartkess A. ^{[2
]}

Wickramasinghe, H. Kumar ^{[4
]}

Potma, Eric Olaf ^{[2
]}

机构：

[1] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA 92697 USA

[2] Univ Calif Irvine, Dept Chem, Irvine, CA 92697 USA

[3] Mol Vista, San Jose, CA 95119 USA

[4] Univ Calif Irvine, Dept Elect Engn & Comp Sci, Irvine, CA 92697 USA

来源：

APPLIED PHYSICS LETTERS | 2015年 / 106卷 / 08期

基金：

美国国家科学基金会;

关键词：

OPTICAL MICROSCOPY; NANOSTRUCTURES; SPECTROSCOPY; ABSORPTION;

D O I：

10.1063/1.4913853

中图分类号：

O59 [应用物理学];

学科分类号：

摘要：

We perform time-resolved pump-probe microscopy measurements by recording the local force between a sharp tip and the photo-excited sample as a readout mechanism for the material's nonlinear polarization. We show that the photo-induced force is sensitive to the same excited state dynamics as measured in an optical pump-probe experiment. Ultrafast pump-probe force microscopy constitutes a non-optical detection technique with nanoscale resolution that pushes pump-probe sensitivities close to the realm of single molecule studies. (C) 2015 AIP Publishing LLC.

引用

页数：4

共 19 条

[1] Ground-State Depletion Microscopy: Detection Sensitivity of Single-Molecule Optical Absorption at Room Temperature [J].

Chong, Shasha ;

Min, Wei ;

Xie, X. Sunney .

JOURNAL OF PHYSICAL CHEMISTRY LETTERS, 2010, 1 (23) :3316-3322

[2] Controlling stimulated coherent spectroscopy and microscopy by a position-dependent phase [J].

Chung, Chao-Yu ;

Hsu, Julie ;

Mukamel, Shaul ;

Potma, Eric O. .

PHYSICAL REVIEW A, 2013, 87 (03)

[3] Coherent nonlinear optical response of single quantum dots studied by ultrafast near-field spectroscopy [J].

Guenther, T ;

Lienau, C ;

Elsaesser, T ;

Glanemann, M ;

Axt, VM ;

Kuhn, T ;

Eshlaghi, S ;

Wieck, AD .

PHYSICAL REVIEW LETTERS, 2002, 89 (05) :057401/1-057401/4

[4] Ultrafast studies of single semiconductor and metal nanostructures through transient absorption microscopy [J].

Hartland, Gregory V. .

CHEMICAL SCIENCE, 2010, 1 (03) :303-309

[5] Nonlinear Optical Microscopy of Single Nanostructures [J].

Huang, Libai ;

Cheng, Ji-Xin .

ANNUAL REVIEW OF MATERIALS RESEARCH, VOL 43, 2013, 43 :213-236

[6] Gradient and scattering forces in photoinduced force microscopy [J].

Jahng, Junghoon ;

Brocious, Jordan ;

Fishman, Dmitry A. ;

Huang, Fei ;

Li, Xiaowei ;

Tamma, Venkata Ananth ;

Wickramasinghe, H. Kumar ;

Potma, Eric Olaf .

PHYSICAL REVIEW B, 2014, 90 (15)

[7] Fast Detection of the Metallic State of Individual Single-Walled Carbon Nanotubes Using a Transient-Absorption Optical Microscope [J].

Jung, Yookyung ;

Slipchenko, Mikhail N. ;

Liu, Chang Hua ;

Ribbe, Alexander E. ;

Zhong, Zhaohui ;

Yang, Chen ;

Cheng, Ji-Xin .

PHYSICAL REVIEW LETTERS, 2010, 105 (21)

[8] Pump-probe scanning near field optical microscopy: Sub-wavelength resolution chemical imaging and ultrafast local dynamics [J].

Karki, Khadga ;

Namboodiri, Mahesh ;

Khan, Tahir Zeb ;

Materny, Arnulf .

APPLIED PHYSICS LETTERS, 2012, 100 (15)

[9] Resonance optical manipulation of nano-objects based on nonlinear optical response [J].

Kudo, Tetsuhiro ;

Ishihara, Hajime .

PHYSICAL CHEMISTRY CHEMICAL PHYSICS, 2013, 15 (35) :14595-14610

[10] Coherent Nonlinear Optical Imaging: Beyond Fluorescence Microscopy [J].

Min, Wei ;

Freudiger, Christian W. ;

Lu, Sijia ;

Xie, X. Sunney .

ANNUAL REVIEW OF PHYSICAL CHEMISTRY, VOL 62, 2011, 62 :507-530

← 1 2 →