Flower-like Nitrogen-co-doped MoS2@RGO Composites with Excellent Stability for Supercapacitors

被引:11
作者
Li, Min [1 ]
Addad, Ahmed [2 ]
Zhang, Yuan [1 ]
Barras, Alexandre [1 ]
Roussel, Pascal [3 ]
Amin, Mohammed A. [4 ]
Szunerits, Sabine [1 ]
Boukherroub, Rabah [1 ]
机构
[1] Univ Lille, Univ Polytech Hauts France, Cent Lille, CNRS,UMR IEMN 8520, F-59000 Lille, France
[2] Univ Lille, CNRS, UMR UMET 8207, F-59000 Lille, France
[3] Univ Lille, Univ Artois, UCCS Unite Catalyse & Chim Solide, Cent Lille,CNRS,ENSCL,UMR 8181, F-59000 Lille, France
[4] Taif Univ, Dept Chem, Coll Sci, POB 11099, At Taif 21944, Saudi Arabia
关键词
molybdenum disulfide; reduced graphene oxide; nitrogen doping; supercapacitors; composites; MOS2-GRAPHENE COMPOSITES; MOS2; NANOSHEETS; GRAPHENE OXIDE; TIO2; NANOTUBES; PERFORMANCE; ELECTRODE; STORAGE; GROWTH; DISULFIDE; DESIGN;
D O I
10.1002/celc.202100401
中图分类号
O646 [电化学、电解、磁化学];
学科分类号
081704 ;
摘要
Nitrogen-co-doped MoS2@rGO composites (named hereafter N-MoS2@N-RGO) are prepared by the hydrothermal method using dicyandiamide or hydrazine monohydrate as the nitrogen source. N-MoS2@rGO is obtained by the hydrothermal reaction of thioacetamide, ammonium molybdate and GO precursors in the presence of dicyandiamide, while N-MoS2@N-RGO is synthesized using the same precursors in the presence of hydrazine monohydrate as the nitrogen source. On the one hand, N-MoS2@RGO displays excellent performance and good capacitance value of 335 F/g acquired at 0.5A/g and improved stability (similar to 94% of the original capacitance is preserved after 5000 cycles). On the other hand, compared with N-MoS2@RGO, N-MoS2@N-RGO possesses a slightly higher capacitance of 340 F/g recorded at 0.5A/g and better cycling stability (similar to 98% of its original value after 5000 cycles). Taken together, the results of this investigation clearly indicate that the fabricated composites have application prospect in energy storage devices.
引用
收藏
页码:2903 / 2911
页数:9
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